Bio-oil from fast pyrolysis of lignin: Effects of process and upgrading parameters

被引：199

作者：

Fan, Liangliang ^{[1
,2
,3
,4
]}

Zhang, Yaning ^{[3
,4
,5
]}

Liu, Shiyu ^{[3
,4
]}

Zhou, Nan ^{[3
,4
]}

Chen, Paul ^{[3
,4
]}

Cheng, Yanling ^{[3
,4
]}

Addy, Min ^{[3
,4
]}

Lu, Qian ^{[3
,4
]}

Omar, Muhammad Mubashar ^{[3
,4
,6
]}

Liu, Yuhuan ^{[1
,2
]}

Wang, Yunpu ^{[2
]}

Dai, Leilei ^{[2
]}

Anderson, Erik ^{[3
,4
]}

Peng, Peng ^{[3
,4
]}

Lei, Hanwu ^{[3
,4
]}

Ruan, Roger ^{[3
,4
]}

机构：

[1] Nanchang Univ, State Key Lab Food Sci & Technol, Nanchang 330047, Jiangxi, Peoples R China

[2] Nanchang Univ, Engn Res Ctr Biomass Convers, Minist Educ, Nanchang 330047, Jiangxi, Peoples R China

[3] Univ Minnesota, Ctr Biorefining, 1390 Eckles Ave, St Paul, MN 55108 USA

[4] Univ Minnesota, Dept Bioprod & Biosyst Engn, 1390 Eckles Ave, St Paul, MN 55108 USA

[5] Harbin Inst Technol, Sch Energy Sci & Engn, Harbin 150001, Peoples R China

[6] Univ Agr Faisalabad, Dept Farm Machinery & Power, Faisalabad, Pakistan

来源：

BIORESOURCE TECHNOLOGY | 2017年 / 241卷

关键词：

Lignin pyrolysis; Bio-oil; Process parameters; Upgrading; CATALYTIC FAST PYROLYSIS; FLUIDIZED-BED REACTOR; LIGNOCELLULOSIC BIOMASS; MICROWAVE PYROLYSIS; CO-PYROLYSIS; ORGANOSOLV LIGNIN; PHENOLIC MONOMERS; METAL-CATALYSTS; HZSM-5; CATALYST; MODEL-COMPOUND;

D O I：

10.1016/j.biortech.2017.05.129

中图分类号：

S2 [农业工程];

学科分类号：

0828 ;

摘要：

Effects of process parameters on the yield and chemical profile of bio-oil from fast pyrolysis of lignin and the processes for lignin-derived bio-oil upgrading were reviewed. Various process parameters including pyrolysis temperature, reactor types, lignin characteristics, residence time, and feeding rate were discussed and the optimal parameter conditions for improved bio-oil yield and quality were concluded. In terms of lignin-derived bio-oil upgrading, three routes including pretreatment of lignin, catalytic upgrading, and co-pyrolysis of hydrogen-rich materials have been investigated. Zeolite cracking and hydrodeoxygenation (HDO) treatment are two main methods for catalytic upgrading of lignin-derived bio-oil. Factors affecting zeolite activity and the main zeolite catalytic mechanisms for lignin conversion were analyzed. Noble metal-based catalysts and metal sulfide catalysts are normally used as the HDO catalysts and the conversion mechanisms associated with a series of reactions have been proposed. (C) 2017 Elsevier Ltd. All rights reserved.

引用

页码：1118 / 1126

页数：9

共 92 条

[1] PRODUCTION OF HYDROCARBONS BY CATALYTIC UPGRADING OF A FAST PYROLYSIS BIO-OIL .2. COMPARATIVE CATALYST PERFORMANCE AND REACTION PATHWAYS [J].