Enhancement of energy storage properties of Bi0.5Na0.5TiO3-based relaxor ferroelectric under moderate electric field

被引:13
作者
Shi, Peng [1 ,2 ]
Hong, Zhengkai [1 ,2 ]
Zhu, Xiaopei [1 ,2 ]
Liu, Qida [3 ]
Yang, Bian [1 ,2 ]
Li, Tangyuan [1 ,2 ]
Kang, Ruirui [1 ,2 ]
Zhao, Jiantuo [1 ,2 ]
Kong, Chuncai [1 ,2 ]
Hu, Yanhua [4 ]
Ke, Xiaoqin [1 ,2 ]
Yang, Sen [1 ,2 ]
Lou, Xiaojie [1 ,2 ]
机构
[1] Xi An Jiao Tong Univ, Frontier Inst Sci & Technol, State Key Lab Mech Behav Mat, Xian 710049, Shaanxi, Peoples R China
[2] Xi An Jiao Tong Univ, Sch Phys, Moe Key Lab Nonequilibrium Synth & Modulat Conden, Xian 710049, Shaanxi, Peoples R China
[3] Xi An Jiao Tong Univ, State Key Lab Strength & Vibrat Mech Structures, Xian 710049, Peoples R China
[4] Ordos Inst Technol, Dept Chem Engn, Ordos 017000, Peoples R China
基金
美国国家科学基金会;
关键词
A-SITE DEFECT; HIGH-EFFICIENCY; GRAIN-SIZE; CERAMICS; DENSITY;
D O I
10.1063/5.0086042
中图分类号
O59 [应用物理学];
学科分类号
摘要
Dielectric capacitors, as one of the important electronic devices, are widely used in various fields. However, most ferroelectric capacitors with high energy storage density require excessively high electric fields. In this work, we have prepared 0.9(Bi0.5Na0.5)(0.7)Sr0.3TiO3-0.1 Bi(Mg2/3Nb1/3)O-3 relaxor ferroelectric ceramics with different BaZrO3 doping levels. A high energy storage (W-r) of 4.07 J/cm(3) and efficiency (eta) of 91% are simultaneously obtained in 0.94[0.9(Bi0.5Na0.5)(0.7)Sr0.3TiO3-0.1 Bi(Mg2/3Nb1/3)O-3]-0.06BaZrO(3) ceramic under a medium electric field of 260 kV/cm. Additionally, the ceramic also exhibits excellent temperature and frequency stability. Furthermore, the phase field simulation is used to simulate the evolution of domain structure and hysteresis loops of the ceramics with different doping levels. The results of phase field simulation explicitly explain the influence of different relaxation degrees on energy storage density and efficiency of the ceramics. We believe that the ceramic prepared in this work is one of the most promising candidate materials for some miniaturized energy storage devices operating under low or medium electric fields. Published under an exclusive license by AIP Publishing.
引用
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页数:8
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