Contamination and Congener Profiles of Polychlorinated Biphenyls from different agricultural top soils in a county of the Tailake Region, China

被引:17
作者
Wang, Hui [1 ]
An, Qiong [1 ]
Dong, Yuan-Hua [1 ]
Li, De-Chen [1 ]
Velde, B. [2 ]
机构
[1] Chinese Acad Sci, Inst Soil Sci, State Key Lab Soil & Sustainable Agr, Nanjing 210008, Peoples R China
[2] Ecole Normale Super, CNRS 4385, Geol Lab, F-75231 Paris, France
关键词
PCBs; Agricultural soils; Different land use types; PERSISTENT ORGANIC POLLUTANTS; SURFACE SOILS; PCBS; LAKE; SEDIMENTS; SHANGHAI; JIANGSU; TAI;
D O I
10.1016/j.jhazmat.2009.11.143
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Hundred topsoil (0-20 cm) samples under different land use types were collected from a county in the Tailake Region, China and analyzed for 18 polychlorinated biphenyls (PCBs) including five dioxin-like PCBs. The mean concentration of total PCBs (Sigma PCBs) for all sites was 1.071 mu g kg(-1) dry weight (dw) with a range of 0.016 mu g kg(-1) to 4.050 mu g kg(-1), and the concentration of total Dioxin-like PCBs (Sigma Dioxin-like PCBs) was 0.352 mu g kg(-1) about 33% of Sigma PCBs. The concentration of Sigma PCBs in paddy field (PF) soils with a mean of 1.637 mu g kg(-1) was higher than that in vegetable soil with a mean of 0.882 mu g kg(-1), but the concentration of Dioxin-like PCBs in PF soil was lower than that in commercial vegetable production soil. The concentration of heavier weighted molecular PCB congeners (>= penta-PCBs) in vegetable soil accounted for 98% of EPCBs, while that in Paddy field soil for 65% of Sigma PCBs. (C) 2009 Elsevier B.V. All rights reserved.
引用
收藏
页码:1027 / 1031
页数:5
相关论文
共 18 条
[1]   Dioxin-like PCBs in the environment - Human exposure and the significance of sources [J].
Alcock, RE ;
Behnisch, PA ;
Jones, KC ;
Hagenmaier, H .
CHEMOSPHERE, 1998, 37 (08) :1457-1472
[2]   PCB in soils and estimated soil-air exchange fluxes of selected PCB congeners in the south of Sweden [J].
Backe, C ;
Cousins, IT ;
Larsson, P .
ENVIRONMENTAL POLLUTION, 2004, 128 (1-2) :59-72
[3]   Polychlorinated biphenyls and their biodegradation [J].
Borja, J ;
Taleon, DM ;
Auresenia, J ;
Gallardo, S .
PROCESS BIOCHEMISTRY, 2005, 40 (06) :1999-2013
[4]   Persistent Toxic Substances in Agricultural Soils of Lishui County, Jiangsu Province, China [J].
Hu, G. -J. ;
Chen, S. -L. ;
Zhao, Y. -G. ;
Sun, C. ;
Li, J. ;
Wang, H. .
BULLETIN OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY, 2009, 82 (01) :48-54
[5]   Preferential sorption of planar contaminants in sediments from Lake Ketelmeer, The Netherlands [J].
Jonker, MTO ;
Smedes, F .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2000, 34 (09) :1620-1626
[6]   Seasonal and spatial character of PCBs in a chemical industrial zone of Shanghai, China [J].
Ma, Jing ;
Cheng, Jinping ;
Xie, Haiyun ;
Hu, Xiaofang ;
Li, Wei ;
Zhang, Jin ;
Yuan, Tao ;
Wang, Wenhua .
ENVIRONMENTAL GEOCHEMISTRY AND HEALTH, 2007, 29 (06) :503-511
[7]   Global distribution and budget of PCBs and HCB in background surface soils: Implications or sources and environmental processes [J].
Meijer, SN ;
Ockenden, WA ;
Sweetman, A ;
Breivik, K ;
Grimalt, JO ;
Jones, KC .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2003, 37 (04) :667-672
[8]   Concentrations and compositions of organochlorine contaminants in sediments, soils, crustaceans, fishes and birds collected from Lake Tai, Hangzhou Bay and Shanghai city region, China [J].
Nakata, H ;
Hirakawa, Y ;
Kawazoe, M ;
Nakabo, T ;
Arizono, K ;
Abe, SI ;
Kitano, T ;
Shimada, H ;
Watanabe, L ;
Li, WH ;
Ding, XC .
ENVIRONMENTAL POLLUTION, 2005, 133 (03) :415-429
[9]   The global re-cycling of persistent organic pollutants is strongly retarded by soils [J].
Ockenden, WA ;
Breivik, K ;
Meijer, SN ;
Steinnes, E ;
Sweetman, AJ ;
Jones, KC .
ENVIRONMENTAL POLLUTION, 2003, 121 (01) :75-80
[10]  
REN M, 2009, CHINA J HAZARD MAT, V170, P473