Identification of nitrogen dioxide and ozone source regions for an urban area in Korea using back trajectory analysis

被引:25
作者
Vellingiri, Kowsalya [1 ]
Kim, Ki-Hyun [1 ]
Lim, Jong-Myoung [2 ]
Lee, Jin-Hong [3 ]
Ma, Chang-Jin [4 ]
Jeon, Byong-Hun [5 ]
Sohn, Jong-Ryeul [6 ]
Kumar, Pawan [7 ]
Kang, Chang-Hee [8 ]
机构
[1] Hanyang Univ, Dept Civil & Environm Engn, 222 Wangsimni Ro, Seoul 04763, South Korea
[2] Korea Atom Energy Res Inst, Environm Radioact Assessment Team, Jeongeup 56212, South Korea
[3] Chungnam Natl Univ, Dept Environm Engn, Taejon 34134, South Korea
[4] Fukuoka Womens Univ, Dept Environm Sci, Fukuoka 8138529, Japan
[5] Hanyang Univ, Dept Nat Resources & Environm Engn, Seoul 04763, South Korea
[6] Korea Univ, Grad Sch, Dept Publ Hlth Sci, Seoul 02708, South Korea
[7] Indian Inst Technol, Dept Chem Engn, Hauz Khas, New Delhi 110016, India
[8] Jeju Natl Univ, Dept Chem, Jeju 63243, South Korea
基金
新加坡国家研究基金会;
关键词
PSCF; Trajectories; Transport; NO2; O-3; GROUND-LEVEL OZONE; LONG-RANGE TRANSPORT; SURFACE OZONE; AIR-POLLUTION; SEOUL; AEROSOL; TRENDS; O-3; METROPOLITAN; REGRESSION;
D O I
10.1016/j.atmosres.2016.02.022
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
The NO2 and O-3 in an urban background site of Seoul, Korea (Yongsan), were analyzed using hourly data collected from 2005 to 2013. The potential role of meteorological parameters in controlling air quality at the receptor site was analyzed using a conditional probability function. In addition, the relative contributions of such variables were examined for special cases (i.e., more than 60 ppb of NO2 and O-3) with the help of trajectory. A potential source contribution function with a grid size resolution of 0.25 degrees x 0.25 degrees was used to determine the potential exogenous sources of NO2 and O-3 for the study area. The results of both the trajectory and potential source contribution function analyses suggest that both the northern China region and local emission sources are the most influential source pathways contributing to the recent increase in NO2 concentration at the study site. In the case of O-3, this role was shared by both oceanic and mountainous regions of China and Japan. (C) 2016 Elsevier B.V. All rights reserved.
引用
收藏
页码:212 / 221
页数:10
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