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Hot corrosion behavior and wettability of calcium-magnesium-alumina-silicate (CMAS) on LaTi2Al9O19 ceramic
被引:49
|作者:
Qu, Weiwei
[1
]
Li, Shusuo
[1
]
Chen, Zehao
[1
]
Li, Chun
[1
]
Pei, Yanling
[1
]
Gong, Shengkai
[1
]
机构:
[1] Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China
基金:
中国国家自然科学基金;
关键词:
LaTi2Al9O19;
ceramic;
Thermodynamic calculation;
Wettability;
Calcium-magnesium-alumina-silicate (CMAS);
Anorthite;
THERMAL BARRIER COATINGS;
Y2O3-STABILIZED ZRO2;
RESISTANT;
MECHANISMS;
AL2O3;
D O I:
10.1016/j.corsci.2019.108199
中图分类号:
T [工业技术];
学科分类号:
08 ;
摘要:
The development of thermal barrier coating (TBC) has been limited by the calcium-magnesium-alumina-silicate (CMAS) corrosion. In this work, a promising CMAS-resisted LaTi2Al9O19 (LTA) rich in Ti and Al is proposed. CMAS corrosion behavior of LTA ceramics is investigated at a temperature range of 1200 degrees C- 1300 degrees C. By combining the experimental results and thermodynamics analysis, Ca and Si are arrested effectively by formation of CaAl2Si2O8 layer and (Ca,La-0.7)(Ti,Al)O-3 to prevent CMAS from moving downward. Meanwhile, the contact angle of CMAS on LTA is larger than that of YSZ, contributing to the CMAS resistance.
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页数:11
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