Influence of the Anthropogenic Fugitive, Combustion, and Industrial Dust on Winter Air Quality in East Asia

被引:5
作者
Jeong, Jaein I. [1 ]
Park, Rokjin J. [1 ]
机构
[1] Seoul Natl Univ, Sch Earth & Environm Sci, Seoul 08826, South Korea
关键词
aerosol; anthropogenic dust; PM10; East Asia; TEMPORAL VARIABILITY; EMISSION INVENTORY; AEROSOL; MODEL; TRANSPORT; POLLUTION; CHINA; PM2.5; SATELLITE; TRENDS;
D O I
10.3390/atmos10120790
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
We estimate the effects of the anthropogenic fugitive, combustion, and industrial dust (AFCID) on winter air quality in China and South Korea for November 2015-March 2016 using the Comprehensive Regional Emissions inventory for Atmospheric Transport Experiment (KU-CREATE) monthly anthropogenic emission inventory in conjunction with a nested version of GEOS-Chem. Including AFCID emissions in models results in a better agreement with observations and a reduced normalized mean bias of -28% compared to -40% without AFCID. Furthermore, we find that AFCID amounts to winter PM10 concentrations of 17.9 mu g m(-3) (17%) in eastern China (30-40 degrees N, 112-120 degrees E) with the largest contribution of AFCID to winter PM10 concentrations of up to 45 mu g m(-3) occurring in eastern China causing a significant impact on air quality to downwind regions. Including AFCID in the model results in an increase of simulated winter PM10 concentrations in South Korea by 3.1 mu g m(-3) (9%), of which transboundary transport from China accounts for more than 70% of this increased PM10 concentration. Our results indicate that AFCID is an essential factor for winter PM10 concentrations over East Asia and its sources and physical characteristics need to be better quantified to improve PM air quality forecasts.
引用
收藏
页数:11
相关论文
共 45 条
  • [1] Sulfate formation in sea-salt aerosols: Constraints from oxygen isotopes
    Alexander, B
    Park, RJ
    Jacob, DJ
    Li, QB
    Yantosca, RM
    Savarino, J
    Lee, CCW
    Thiemens, MH
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2005, 110 (D10) : 1 - 12
  • [2] Chin M, 2002, J ATMOS SCI, V59, P461, DOI 10.1175/1520-0469(2002)059<0461:TAOTFT>2.0.CO
  • [3] 2
  • [4] Impacts of local vs. trans-boundary emissions from different sectors on PM2.5 exposure in South Korea during the KORUS-AQ campaign
    Choi, Jinkyul
    Park, Rokjin J.
    Lee, Hyung-Min
    Lee, Seungun
    Jo, Duseong S.
    Jeong, Jaein I.
    Henze, Daven K.
    Woo, Jung-Hun
    Ban, Soo-Jin
    Lee, Min-Do
    Lim, Cheol-Soo
    Park, Mi-Kyung
    Shin, Hye J.
    Cho, Seogju
    Peterson, David
    Song, Chang-Keun
    [J]. ATMOSPHERIC ENVIRONMENT, 2019, 203 : 196 - 205
  • [5] Cohen AJ, 2017, LANCET, V389, P1907, DOI [10.1016/S0140-6736(17)30505-6, 10.1016/s0140-6736(17)30505-6]
  • [6] The impact of transpacific transport of mineral dust in the United States
    Fairlie, T. Duncan
    Jacob, Daniel J.
    Park, Rokjin J.
    [J]. ATMOSPHERIC ENVIRONMENT, 2007, 41 (06) : 1251 - 1266
  • [7] ISORROPIA II:: a computationally efficient thermodynamic equilibrium model for K+-Ca2+-Mg2+-Nh4+-Na+-SO42--NO3--Cl--H2O aerosols
    Fountoukis, C.
    Nenes, A.
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (17) : 4639 - 4659
  • [8] Analysis of daily, monthly, and annual burned area using the fourth-generation global fire emissions database (GFED4)
    Giglio, Louis
    Randerson, James T.
    van der Werf, Guido R.
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES, 2013, 118 (01) : 317 - 328
  • [9] Sources and distributions of dust aerosols simulated with the GOCART model
    Ginoux, P
    Chin, M
    Tegen, I
    Prospero, JM
    Holben, B
    Dubovik, O
    Lin, SJ
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D17) : 20255 - 20273
  • [10] A parameterization of sea-salt aerosol source function for sub- and super-micron particles
    Gong, SL
    [J]. GLOBAL BIOGEOCHEMICAL CYCLES, 2003, 17 (04)