Low-cost reed straw-derived biochar prepared by hydrothermal carbonization for the removal of uranium(VI) from aqueous solution

被引:15
|
作者
Liu, Yuting [2 ]
Wang, Yun [1 ,2 ]
Xia, Hongtao [2 ]
Wang, Qinghua [2 ]
Chen, Xinchen [2 ]
Lv, Jianqi [2 ]
Li, Yang [2 ]
Zhao, Jiankun [1 ,2 ]
Liu, Yan [3 ]
Yuan, Dingzhong [3 ]
机构
[1] East China Univ Technol, Minist Educ, Engn Res Ctr Nucl Technol Applicat, Nanchang 330013, Jiangxi, Peoples R China
[2] East China Univ Technol, Sch Nucl Sci & Engn, Nanchang 330013, Jiangxi, Peoples R China
[3] East China Univ Technol, Sch Chem Biol & Mat Sci, Nanchang 330013, Jiangxi, Peoples R China
基金
中国国家自然科学基金;
关键词
Uranium; Adsorption; Biochar; Reed straw; Hydrothermal carbonization; KOH ACTIVATION; CARBON SPHERES; ADSORPTION; HYDROCHAR; SLUDGE; U(VI);
D O I
10.1007/s10967-022-08421-y
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Uranium is the important nuclear fuel and its effective adsorption using low-cost materials is meaningful to environmental protection and sustainable development of nuclear energy. In this study, green and economical reed straw-derived biochar (RBC) was prepared by hydrothermal carbonization method using low-cost reed straw as feedstocks and citric acid as catalysts for uranium(VI) removal. RBC possessed larger pores and more oxygen-containing functional groups, providing more abundant adsorption sites for uranyl ions. RBC adsorbed uranium pH-dependently, spontaneously and endothermically, and pseudo-second-order kinetics and the Langmuir model could adequately describe the adsorption process. This work highlighted a feasible synthesis strategy of biochar for radioactive contaminants removal.
引用
收藏
页码:3915 / 3925
页数:11
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