75As nuclear magnetic resonance study of antiferromagnetic fluctuations in the normal state of LiFeAs

被引:49
作者
Jeglic, P. [1 ]
Potocnik, A. [1 ]
Klanjsek, M. [1 ]
Bobnar, M. [1 ]
Jagodic, M. [2 ]
Koch, K. [3 ]
Rosner, H. [3 ]
Margadonna, S. [4 ]
Lv, B. [5 ,6 ]
Guloy, A. M. [5 ,6 ]
Arcon, D. [1 ,7 ]
机构
[1] Jozef Stefan Inst, Ljubljana 1000, Slovenia
[2] Inst Math Phys & Mech, Ljubljana 1000, Slovenia
[3] Max Planck Inst Chem Phys Fester Stoffe, D-01187 Dresden, Germany
[4] Univ Edinburgh, Sch Chem, Edinburgh EH9 3JJ, Midlothian, Scotland
[5] Univ Houston, Dept Chem, Houston, TX 77204 USA
[6] Univ Houston, TCSUH, Houston, TX 77204 USA
[7] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia
关键词
NMR; SUPERCONDUCTOR; YBA2CU3O7; MODEL;
D O I
10.1103/PhysRevB.81.140511
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We present a detailed study of As-75 nuclear magnetic resonance Knight shift and spin-lattice relaxation rate in the normal state of stoichiometric polycrystalline LiFeAs. Our analysis of the Korringa relation suggests that LiFeAs exhibits strong antiferromagnetic fluctuations, if transferred hyperfine coupling is a dominant interaction between As-75 nuclei and Fe electronic spins, whereas for an on-site hyperfine coupling scenario, these are weaker, but still present to account for our experimental observations. Density-functional calculations of electric field gradient correctly reproduce the experimental values for both As-75 and Li-7 sites.
引用
收藏
页数:4
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