Preparation and characterization of Ag-doped TiO2 nanomaterials and their photocatalytic reduction of Cr(VI) under visible light

被引：191
作者：
Lei, X. F. [1 ,2 ,3 ,4 ,5 ]
Xue, X. X. [2 ,3 ,4 ,5 ]
Yang, H. [2 ,3 ,4 ,5 ]
机构：
[1] Northeastern Univ Qinhuangdao, Sch Resources & Mat, Qinhuangdao 066004, Peoples R China
[2] Northeastern Univ, Inst Met Resource & Environm Engn, Shenyang 110819, Peoples R China
[3] Liaoning Key Lab Met Resource Recycling Sci, Shenyang 110819, Peoples R China
[4] Liaoning Engn & Technol Res Ctr Boron Resource, Shenyang 110819, Peoples R China
[5] Liaoning Prov Univ Key Lab Boron Resource Ecol Ut, Shenyang 110819, Peoples R China
来源：
APPLIED SURFACE SCIENCE | 2014年 / 321卷
关键词：
Ag-doped; TiO2; Calcination temperature; Photocatalytic activity; Visible light; Cr(VI); SURFACE-AREA; DEGRADATION; TITANIA; SILVER; OXIDE; NANOPARTICLES; PERFORMANCE; ADSORPTION; WATER;
D O I：
10.1016/j.apsusc.2014.10.045
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Ag-doped TiO2 nanomaterials (Ag-TiO2) were prepared by a sol-gel method. The structures of Ag-TiO2 nanomaterials were characterized by X-ray diffraction (XRD), UV-vis diffuse reflectance spectra (DRS), X-ray photoluminescence (PL) spectroscopy, X-ray photoelectron spectroscopy (XPS), thermogravimetry and differential thermal analysis (TG-DTA), Fourier transform infrared spectroscopy (FT-IR), transmission electron microscope (TEM), scanning electron microscopy (SEM) and nitrogen adsorption-desorption isotherms. The photocatalytic activities were checked through the photocatalytic reduction of Cr(VI) as a model compound under visible light irradiation. The results showed that the Ag doping and the calcination temperature played an important role on the microstructure and photocatalytic activity of the samples. Ag-doped TiO2 samples calcinated at 400 degrees C exhibits higher photocatalytic activity than that of the other samples under visible light irradiation. (C) 2014 Elsevier B.V. All rights reserved.
引用
收藏
页码：396 / 403
页数：8
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