Formation of secondary organic aerosols from anthropogenic precursors in laboratory studies

被引：106
|
作者：
Srivastava, Deepchandra [1 ]
Vu, Tuan V. [2 ]
Tong, Shengrui [3 ,4 ]
Shi, Zongbo [1 ]
Harrison, Roy M. [1 ,5 ]
机构：
[1] Univ Birmingham, Sch Geog Earth & Environm Sci, Div Environm Hlth & Risk Management, Birmingham B15 2TT, W Midlands, England
[2] Imperial Coll London, Fac Med, Sch Publ Hlth, London, England
[3] Chinese Acad Sci Zhongguancun, State Key Lab Struct Chem Unstable, Beijing 100190, Peoples R China
[4] Chinese Acad Sci Zhongguancun, Stable Species Inst Chem, Beijing 100190, Peoples R China
[5] King Abdulaziz Univ, Ctr Excellence Environm Studies, Dept Environm Sci, POB 80203, Jeddah 21589, Saudi Arabia
来源：
NPJ CLIMATE AND ATMOSPHERIC SCIENCE | 2022年 / 5卷 / 01期
基金：
英国自然环境研究理事会;
关键词：
POLYCYCLIC AROMATIC-HYDROCARBONS; GAS-PHASE REACTIONS; RADICAL-INITIATED REACTIONS; HIGH-NOX PHOTOOXIDATION; SPECTROMETER EESI-TOF; LOW-VOLATILITY ORGANICS; AIR-POLLUTION SOURCES; LONG-CHAIN ALKANES; SOA FORMATION; CHEMICAL-COMPOSITION;
D O I：
10.1038/s41612-022-00238-6
中图分类号：
P4 [大气科学（气象学）];
学科分类号：
0706 ; 070601 ;
摘要：
Aerosols produced from the oxidation of volatile/semi-volatile organic compounds (VOCs/SVOCs), known as secondary organic aerosol (SOA), account for a significant fraction of atmospheric airborne particles. This paper reviews the current understanding of SOA formation from gas-phase oxidation with a focus on anthropogenic precursors and their reaction products from atmospheric simulation chamber studies. The review summarises the major reaction products derived from main groups of SOA precursors (e.g., alkanes, aromatics), SOA yields and the factors controlling SOA formation. We highlight that lab-derived SOA yield depends strongly upon, not only the concentrations of SOA precursors and oxidants but also simulation conditions.
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页数：30
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