Formation of secondary organic aerosols from anthropogenic precursors in laboratory studies

被引：132

作者：

Srivastava, Deepchandra ^{[1
]}

Vu, Tuan V. ^{[2
]}

Tong, Shengrui ^{[3
,4
]}

Shi, Zongbo ^{[1
]}

Harrison, Roy M. ^{[1
,5
]}

机构：

[1] Univ Birmingham, Sch Geog Earth & Environm Sci, Div Environm Hlth & Risk Management, Birmingham B15 2TT, W Midlands, England

[2] Imperial Coll London, Fac Med, Sch Publ Hlth, London, England

[3] Chinese Acad Sci Zhongguancun, State Key Lab Struct Chem Unstable, Beijing 100190, Peoples R China

[4] Chinese Acad Sci Zhongguancun, Stable Species Inst Chem, Beijing 100190, Peoples R China

[5] King Abdulaziz Univ, Ctr Excellence Environm Studies, Dept Environm Sci, POB 80203, Jeddah 21589, Saudi Arabia

来源：

NPJ CLIMATE AND ATMOSPHERIC SCIENCE | 2022年 / 5卷 / 01期

基金：

英国自然环境研究理事会;

关键词：

POLYCYCLIC AROMATIC-HYDROCARBONS; GAS-PHASE REACTIONS; RADICAL-INITIATED REACTIONS; HIGH-NOX PHOTOOXIDATION; SPECTROMETER EESI-TOF; LOW-VOLATILITY ORGANICS; AIR-POLLUTION SOURCES; LONG-CHAIN ALKANES; SOA FORMATION; CHEMICAL-COMPOSITION;

D O I：

10.1038/s41612-022-00238-6

中图分类号：

P4 [大气科学（气象学）];

学科分类号：

0706 ; 070601 ;

摘要：

Aerosols produced from the oxidation of volatile/semi-volatile organic compounds (VOCs/SVOCs), known as secondary organic aerosol (SOA), account for a significant fraction of atmospheric airborne particles. This paper reviews the current understanding of SOA formation from gas-phase oxidation with a focus on anthropogenic precursors and their reaction products from atmospheric simulation chamber studies. The review summarises the major reaction products derived from main groups of SOA precursors (e.g., alkanes, aromatics), SOA yields and the factors controlling SOA formation. We highlight that lab-derived SOA yield depends strongly upon, not only the concentrations of SOA precursors and oxidants but also simulation conditions.

引用

页数：30

共 238 条

[1] Particulate Matter Air Pollution and Cardiovascular Disease An Update to the Scientific Statement From the American Heart Association [J].

Brook, Robert D. ;

Rajagopalan, Sanjay ;

Pope, C. Arden, III ;

Brook, Jeffrey R. ;

Bhatnagar, Aruni ;

Diez-Roux, Ana V. ;

Holguin, Fernando ;

Hong, Yuling ;

Luepker, Russell V. ;

Mittleman, Murray A. ;

Peters, Annette ;

Siscovick, David ;

Smith, Sidney C., Jr. ;

Whitsel, Laurie ;

Kaufman, Joel D. .

CIRCULATION, 2010, 121 (21) :2331-2378

[2] Production of Secondary Organic Aerosol During Aging of Biomass Burning Smoke From Fresh Fuels and Its Relationship to VOC Precursors [J].

Ahern, A. T. ;

Robinson, E. S. ;

Tkacik, D. S. ;

Saleh, R. ;

Hatch, L. E. ;

Barsanti, K. C. ;

Stockwell, C. E. ;

Yokelson, R. J. ;

Presto, A. A. ;

Robinson, A. L. ;

Sullivan, R. C. ;

Donahue, N. M. .

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2019, 124 (06) :3583-3606

[3] Chemical Mechanisms of Aging of Aerosol Formed from the Reaction of n-Pentadecane with OH Radicals in the Presence of NOx [J].

Aimanant, Sukon ;

Ziemann, Paul J. .

AEROSOL SCIENCE AND TECHNOLOGY, 2013, 47 (09) :979-990

[4] Mapping and quantifying isomer sets of hydrocarbons ( ≥ C12) in diesel exhaust, lubricating oil and diesel fuel samples using GC x GC-ToF-MS [J].

Alam, Mohammed S. ;

Zeraati-Rezaei, Soheil ;

Liang, Zhirong ;

Stark, Christopher ;

Xu, Hongming ;

MacKenzie, A. Rob ;

Harrison, Roy M. .

ATMOSPHERIC MEASUREMENT TECHNIQUES, 2018, 11 (05) :3047-3058

[5] Secondary organic aerosol formation in northern Europe:: A model study [J].

Andersson-Sköld, Y ;

Simpson, D .

JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2001, 106 (D7) :7357-7374

[6]

[Anonymous], 2014, The Physical Science Ba- sis: Working Group I Contribution to the Fifth Assessment Re- port of the Intergovernmental Panel on Climate Change, DOI [10.1017/CBO9781107415324, DOI 10.1017/CBO9781107415324]

[7] Dicarbonyl Products of the OH Radical-Initiated Reaction of a Series of Aromatic Hydrocarbons [J].

Arey, Janet ;

Obermeyer, Genevieve ;

Aschmann, Sara M. ;

Chattopadhyay, Sulekha ;

Cusick, Roland D. ;

Atkinson, Roger .

ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2009, 43 (03) :683-689

[8] Polar sunrise experiment 1995: Hydrocarbon measurements and tropospheric Cl and Br-atoms chemistry [J].

Ariya, PA ;

Niki, H ;

Harris, GW ;

Anlauf, KG ;

Worthy, DEJ .

ATMOSPHERIC ENVIRONMENT, 1999, 33 (06) :931-938

[9] Extent of H-atom abstraction from OH plus p-cymene and upper limits to the formation of cresols from OH plus m-xylene and OH plus p-cymene [J].

Aschmann, Sara M. ;

Arey, Janet ;

Atkinson, Roger .

ATMOSPHERIC ENVIRONMENT, 2010, 44 (32) :3970-3975

[10] Gas-phase tropospheric chemistry of volatile organic compounds .1. Alkanes and alkenes [J].

Atkinson, R .

JOURNAL OF PHYSICAL AND CHEMICAL REFERENCE DATA, 1997, 26 (02) :215-290

← 1 2 3 4 5 6 7 8 9 10 →