Regional atmospheric emissions determined from measurements at Jeju Island, Korea: Halogenated compounds from China

被引:86
作者
Kim, Jooil [1 ]
Li, Shanlan [1 ]
Kim, Kyung -Ryul [1 ,2 ]
Stohl, Andreas [3 ]
Muehle, Jens [4 ]
Kim, Seung -Kyu [1 ]
Park, Mi -Kyung [1 ,2 ]
Kang, Dong -Jin [5 ]
Lee, Gangwoong [6 ]
Harth, Christina M. [4 ]
Salameh, Peter K. [4 ]
Weiss, Ray F. [4 ]
机构
[1] Seoul Natl Univ, Sch Earth & Environm Sci, Seoul 151747, South Korea
[2] Seoul Natl Univ, Res Inst Oceanog, Seoul 151747, South Korea
[3] Norwegian Inst Air Res, N-2027 Kjeller, Norway
[4] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA
[5] Korea Ocean Res & Dev Inst, Seoul 426744, South Korea
[6] Hankuk Univ Foreign Studies, Div Environm Sci, Yongin 449741, Gyeonggido, South Korea
关键词
GLOBAL EMISSIONS; GASES; ASIA;
D O I
10.1029/2010GL043263
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
High-frequency in-situ measurements of a wide range of halogenated compounds including chlorofluorocarbons (CFCs), halons, hydrochlorofluorocarbons (HCFCs), hydrofluorocarbons (HFCs), perfluorinated compounds (PFCs), sulfur hexafluoride (SF6), and other chlorinated and brominated compounds have been made at Gosan (Jeju Island, Korea). Regional emissions of HCFC-22 (CHClF2) calculated from inverse modeling were combined with interspecies correlation methods to estimate national emissions for China, a major emitter of industrial halogenated gases. Our results confirm the signs of successful phase-out of primary ozone-depleting species such as CFCs, halons and many chlorinated or brominated compounds, along with substantial emissions of replacement HCFCs. Emissions derived for HFCs, PFCs, and SF6 were compared to published estimates and found to be a significant fraction of global totals. Overall, Chinese emissions of the halogenated compounds discussed here represent 19(14-17)% and 20(15-26)% of global emissions when evaluated in terms of their Ozone Depletion Potentials and 100-year Global Warming Potentials, respectively. Citation: Kim, J., et al. (2010), Regional atmospheric emissions determined from measurements at Jeju Island, Korea: Halogenated compounds from China, Geophys. Res. Lett., 37, L12801, doi: 10.1029/2010GL043263.
引用
收藏
页数:5
相关论文
共 24 条
  • [1] [Anonymous], ATMOS CHEM PHYS
  • [2] [Anonymous], 2009, HDB MONTR PROT SUBST, VEighth
  • [3] Surface aerosol radiative forcing at Gosan during the ACE-Asia campaign
    Bush, BC
    Valero, FPJ
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D23)
  • [4] CLERBAUX C, 2007, SCI ASSESSMENT OZONE, V50
  • [5] EDGAR, 2009, EM DAT GLOB ATM RES
  • [6] Forster P, 2007, AR4 CLIMATE CHANGE 2007: THE PHYSICAL SCIENCE BASIS, P129
  • [7] [胡建信 Hu Jianxin], 2009, [气候变化研究进展, Advances in Climate Change Research], V5, P1
  • [8] The global SF6 source inferred from long-term high precision atmospheric measurements and its comparison with emission inventories
    Levin, I.
    Naegler, T.
    Heinz, R.
    Osusko, D.
    Cuevas, E.
    Engel, A.
    Ilmberger, J.
    Langenfelds, R. L.
    Neininger, B.
    Von Rohden, C.
    Steele, L. P.
    Weller, R.
    Worthy, D. E.
    Zimov, S. A.
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2010, 10 (06) : 2655 - 2662
  • [9] Global emissions of HFC-23 estimated to year 2015
    McCulloch, A.
    Lindley, A. A.
    [J]. ATMOSPHERIC ENVIRONMENT, 2007, 41 (07) : 1560 - 1566
  • [10] Medusa: A sample preconcentration and GC/MS detector system for in situ measurements of atmospheric trace halocarbons, hydrocarbons, and sulfur compounds
    Miller, Benjamin R.
    Weiss, Ray F.
    Salameh, Peter K.
    Tanhua, Toste
    Greally, Brian R.
    Muhle, Jens
    Simmonds, Peter G.
    [J]. ANALYTICAL CHEMISTRY, 2008, 80 (05) : 1536 - 1545