1T/1T′-dominated WSe2 with stabilized oxygen dopants for efficient and durable hydrogen evolution

被引:9
作者
Sun, Zhuxing [1 ]
Wang, Yiwen [1 ]
Lang, Junyu [1 ]
Yang, Mengfei [1 ]
Jin, Fangming [1 ]
Hu, Yun Hang [2 ]
机构
[1] Shanghai Jiao Tong Univ, Sch Environm Sci & Engn, Shanghai 200240, Peoples R China
[2] Michigan Technol Univ, Dept Mat Sci & Engn, Houghton, MI 49931 USA
基金
中国国家自然科学基金;
关键词
TRANSITION-METAL DICHALCOGENIDES; HIGHLY EFFICIENT; 1T PHASE; STABLE ELECTROCATALYST; NANOSHEETS; MOS2; ELECTRODE;
D O I
10.1039/d1ta01370j
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
For the first time, the importance of the oxidized W species in WSe2 catalysts for HER is revealed. Meanwhile, via a specifically designed yet facile solvothermal strategy, a 1T/1T ' dominated hybrid-phase WSe2 with stabilized oxygen species was obtained, realizing outstanding activity and durability for HER.
引用
收藏
页码:13490 / 13495
页数:6
相关论文
共 43 条
[1]   2H → 1T phase transition and hydrogen evolution activity of MoS2, MoSe2, WS2 and WSe2 strongly depends on the MX2 composition [J].
Ambrosi, Adriano ;
Sofer, Zdenek ;
Pumera, Martin .
CHEMICAL COMMUNICATIONS, 2015, 51 (40) :8450-8453
[2]   Solution synthesis of few-layer 2H MX2 (M = Mo, W; X = S, Se) [J].
Barrera, Diego ;
Wang, Qingxiao ;
Lee, Yun-Ju ;
Cheng, Lanxia ;
Kim, Moon J. ;
Kim, Jiyoung ;
Hsu, Julia W. P. .
JOURNAL OF MATERIALS CHEMISTRY C, 2017, 5 (11) :2859-2864
[3]   Hydrogen: A brief overview on its sources, production and environmental impact [J].
Baykara, Sema Z. .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2018, 43 (23) :10605-10614
[4]   1T Phase Transition Metal Dichalcogenides for Hydrogen Evolution Reaction [J].
Chang, Liang ;
Sun, Zhuxing ;
Hu, Yun Hang .
ELECTROCHEMICAL ENERGY REVIEWS, 2021, 4 (02) :194-218
[5]   Large quantum-spin-Hall gap in single-layer 1T′ WSe2 [J].
Chen, P. ;
Pai, Woei Wu ;
Chan, Y. -H. ;
Sun, W. -L. ;
Xu, C. -Z. ;
Lin, D. -S. ;
Chou, M. Y. ;
Fedorov, A. -V. ;
Chiang, T. -C. .
NATURE COMMUNICATIONS, 2018, 9
[6]   Emerging two-dimensional nanomaterials for electrochemical hydrogen evolution [J].
Chen, Yunxu ;
Yang, Kena ;
Jiang, Bei ;
Li, Jiaxu ;
Zeng, Mengqi ;
Fu, Lei .
JOURNAL OF MATERIALS CHEMISTRY A, 2017, 5 (18) :8187-8208
[7]   Memristive Behavior and Ideal Memristor of 1T Phase MoS2 Nanosheets [J].
Cheng, Peifu ;
Sun, Kai ;
Hu, Yun Hang .
NANO LETTERS, 2016, 16 (01) :572-576
[8]  
Chhowalla M, 2013, NAT CHEM, V5, P263, DOI [10.1038/NCHEM.1589, 10.1038/nchem.1589]
[9]   Morphological Effects and Stabilization of the Metallic 1T Phase in Layered V-, Nb-, and Ta-Doped WSe2 for Electrocatalysis [J].
Chia, Xinyi ;
Sutrisnoh, Nur Ayu Afira ;
Sofer, Zdenek ;
Luxa, Jan ;
Pumera, Martin .
CHEMISTRY-A EUROPEAN JOURNAL, 2018, 24 (13) :3199-3208
[10]   Catalytic and Charge Transfer Properties of Transition Metal Dichalcogenides Arising from Electrochemical Pretreatment [J].
Chia, Xinyi ;
Ambrosi, Adriano ;
Sofer, Zdenek ;
Luxa, Jan ;
Pumera, Martin .
ACS NANO, 2015, 9 (05) :5164-5179