Highly efficient photoelectrochemical anticorrosion performance of C3N4@ZnO composite with quasi-shell-core structure on 304 stainless steel

被引:53
作者
Bu, Yuyu [1 ]
Chen, Zhuoyuan [1 ]
机构
[1] Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, Qingdao 266071, Peoples R China
基金
中国国家自然科学基金;
关键词
CORROSION PROTECTION; HYDROGEN-PRODUCTION; THIN-FILM; ZNO; COATINGS; PHOTOCATALYST; SRTIO3; STEEL; WATER;
D O I
10.1039/c4ra06641c
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Carbon nitride@zinc oxide (C3N4@ZnO) composite with a quasi-shell-core structure was prepared in this work. The coating of C3N4 on ZnO significantly increases the photoelectrochemical anticorrosion performance of ZnO. When the amount of C3N4 added is 1 wt%, the C3N4@ZnO composite can provide the best photoelectrochemical anticorrosion capability for 304 stainless steel. This improved performance is attributed to the formation of an effective heterojunction electric field on the interface between C3N4 and ZnO, which improves the separation efficiency of the photogenerated electron-hole pairs, increases the lifetime of the photoinduced electrons, and enhances the photoelectrochemical anticorrosion performance of ZnO.
引用
收藏
页码:45397 / 45406
页数:10
相关论文
共 27 条
[1]   Fabrication of SrTiO3 Nanocrystalline Film Photoelectrode and Its Photoelectrochemical Anticorrosion Properties for Stainless Steel [J].
Bu Yu-Yu ;
Li Wei-Bing ;
Yu Jian-Qiang ;
Wang Xiu-Tong ;
Qi Mei-Ling ;
Nie Meng-Yan ;
Hou Bao-Rong .
ACTA PHYSICO-CHIMICA SINICA, 2011, 27 (10) :2393-2399
[2]   Highly Efficient Photocatalytic Performance of Graphene-ZnO Quasi-Shell-Core Composite Material [J].
Bu, Yuyu ;
Chen, Zhuoyuan ;
Li, Weibing ;
Hou, Baorong .
ACS APPLIED MATERIALS & INTERFACES, 2013, 5 (23) :12361-12368
[3]   A novel application of g-C3N4 thin film in photoelectrochemical anticorrosion [J].
Bu, Yuyu ;
Chen, Zhuoyuan ;
Yu, Jianqiang ;
Li, Weibing .
ELECTROCHIMICA ACTA, 2013, 88 :294-300
[4]   Preparation of the new polyaniline/ZnO nanocomposite and its photocatalytic activity for degradation of methylene blue and malachite green dyes under UV and natural sun lights irradiations [J].
Eskizeybek, Volkan ;
Sari, Fahriye ;
Gulce, Handan ;
Gulce, Ahmet ;
Avci, Ahmet .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2012, 119 :197-206
[5]   Chemical synthesis of mesoporous carbon nitrides using hard templates and their use as a metal-free catalyst for friedel-crafts reaction of benzene [J].
Goettmann, Frederic ;
Fischer, Anna ;
Antonietti, Markus ;
Thomas, Arne .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2006, 45 (27) :4467-4471
[6]   Photogenerated cathodic protection of stainless steel by liquid-phase-deposited sodium polyacrylate/TiO2 hybrid films [J].
Lei, Caixia ;
Liu, Yu ;
Zhou, Han ;
Feng, Zude ;
Du, Ronggui .
CORROSION SCIENCE, 2013, 68 :214-222
[7]   Improvement in corrosion protection properties of TiO2 coatings by chromium doping [J].
Li, Suning ;
Fu, Jiajun .
CORROSION SCIENCE, 2013, 68 :101-110
[8]   Study on cerium-doped nano-TiO2 coatings for corrosion protection of 316 L stainless steel [J].
Li, Suning ;
Wang, Qian ;
Chen, Tao ;
Zhou, Zhihua ;
Wang, Ying ;
Fu, Jiajun .
NANOSCALE RESEARCH LETTERS, 2012, 7
[9]   A highly efficient ZnS/CdS@TiO2 photoelectrode for photogenerated cathodic protection of metals [J].
Lin, Ze-Quan ;
Lai, Yue-Kun ;
Hu, Rong-Gang ;
Li, Jing ;
Du, Rong-Gui ;
Lin, Chang-Jian .
ELECTROCHIMICA ACTA, 2010, 55 (28) :8717-8723
[10]   Photoelectrochemical anticorrosion effect of SrTiO3 for carbon steel [J].
Ohko, Y ;
Saitoh, S ;
Tatsuma, T ;
Fujishima, A .
ELECTROCHEMICAL AND SOLID STATE LETTERS, 2002, 5 (02) :B9-B12