Scalable top-down synthesis of functional carbon nanosheets by aronia fruit powder for Li+ and K+ storage

被引:6
作者
Cheong, Jun Young [1 ,4 ]
Jung, Ji-Won [1 ,2 ]
Kim, Chanhoon [3 ]
Kim, Il-Doo [1 ]
机构
[1] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, 335 Sci Rd, Daejeon 305701, South Korea
[2] Univ Ulsan, Sch Mat Sci & Engn, Techno Saneop Ro 55, Ulsan 44776, South Korea
[3] Korea Inst Ind Technol, Sustainable Technol & Wellness R&D Grp, 102 Jejudaehak Ro, Jeju Si 63243, Jeju Do, South Korea
[4] Samsung SDI, 467 Beonyeong Ro, Cheonan 31086, South Korea
基金
新加坡国家研究基金会;
关键词
Carbon; Nanosheet; Lithium; Potassium; Aronia; Battery; THERMOOXIDATIVE DEGRADATION; ANODE MATERIALS; POTASSIUM-ION; LITHIUM; GRAPHENE; ENERGY; MELANOCARPA; NANOFIBERS; COMPOSITES; GRAPHITE;
D O I
10.1016/j.electacta.2021.138068
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
Carbon nanosheets (CNSs) have been used in various applications, ranging from energy storage to drug delivery. CNSs are conventionally synthesized by chemical vapor deposition, but their high cost and non-scalability prompted the development of alternative synthesis routes. More scalable methods such as the sol-gel process still suffer from its complicated synthetic steps with delicate conditions. Here, we demonstrate for the first time a unique top-down synthesis of CNSs from aronia fruit powder, which is simple, scalable, and cost-effective. Aronia-derived CNS can be fabricated at various heating temperatures (500, 700, and 90 0 degrees C) and under different atmospheres (N-2/H-2 and NH3), which can easily tune the overall physicochemical properties of the CNS. We evaluated the electrochemical performance of the CNS for potential applications in Li- and K-ion batteries, in which the CNS showed stable electrochemical performance even at a high current density (1000 mA g(-1)). Because of the high-throughput nature of this synthetic approach, the aronia-derived CNSs could be very useful in developing novel applications at an industrial scale. (C) 2021 Published by Elsevier Ltd.
引用
收藏
页数:10
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