Electron turbulence at nanoscale junctions

被引:12
作者
Bushong, Neil [1 ]
Gamble, John
Di Ventra, Massimiliano
机构
[1] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA
[2] Coll Wooster, Dept Phys, Wooster, OH 44691 USA
关键词
D O I
10.1021/nl070935e
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Electron transport through a nanostructure can be characterized in part using concepts from classical fluid dynamics. It is thus natural to ask how far the analogy can be taken and whether the electron liquid can exhibit nonlinear dynamical effects such as turbulence. Here we present an ab initio study of the electron dynamics in nanojunctions which reveals that the latter indeed exhibits behavior quite similar to that of a classical fluid. In particular, we find that a transition from laminar to turbulent flow occurs with increasing current, corresponding to increasing Reynolds numbers. These results reveal unexpected features of electron dynamics and shed new light on our understanding of transport properties of nanoscale systems.
引用
收藏
页码:1789 / 1792
页数:4
相关论文
共 35 条
[21]   THEORY OF MANY-PARTICLE SYSTEMS .1. [J].
MARTIN, PC ;
SCHWINGER, J .
PHYSICAL REVIEW, 1959, 115 (06) :1342-1373
[22]  
Palacios JJ, 2002, PHYS REV B, V66, DOI 10.1103/PhysRevB.66.035322
[23]   SELF-INTERACTION CORRECTION TO DENSITY-FUNCTIONAL APPROXIMATIONS FOR MANY-ELECTRON SYSTEMS [J].
PERDEW, JP ;
ZUNGER, A .
PHYSICAL REVIEW B, 1981, 23 (10) :5048-5079
[24]   Gerris: a tree-based adaptive solver for the incompressible Euler equations in complex geometries [J].
Popinet, S .
JOURNAL OF COMPUTATIONAL PHYSICS, 2003, 190 (02) :572-600
[25]   Benchmarking the performance of density functional theory based Green's function formalism utilizing different self-energy models in calculating electronic transmission through molecular systems [J].
Prociuk, Alexander ;
Van Kuiken, Ben ;
Dunietz, Barry D. .
JOURNAL OF CHEMICAL PHYSICS, 2006, 125 (20)
[26]   DENSITY-FUNCTIONAL THEORY FOR TIME-DEPENDENT SYSTEMS [J].
RUNGE, E ;
GROSS, EKU .
PHYSICAL REVIEW LETTERS, 1984, 52 (12) :997-1000
[27]   Microscopic current dynamics in nanoscale junctions [J].
Sai, Na ;
Bushong, Neil ;
Hatcher, Ryan ;
Di Ventra, Massimiliano .
PHYSICAL REVIEW B, 2007, 75 (11)
[28]   The high-bias stability of monatomic chains [J].
Smit, RHM ;
Untiedt, C ;
van Ruitenbeek, JM .
NANOTECHNOLOGY, 2004, 15 (07) :S472-S478
[29]   AN ACCURATE AND EFFICIENT SCHEME FOR PROPAGATING THE TIME-DEPENDENT SCHRODINGER-EQUATION [J].
TALEZER, H ;
KOSLOFF, R .
JOURNAL OF CHEMICAL PHYSICS, 1984, 81 (09) :3967-3971
[30]   Ab initio modeling of quantum transport properties of molecular electronic devices -: art. no. 245407 [J].
Taylor, J ;
Guo, H ;
Wang, J .
PHYSICAL REVIEW B, 2001, 63 (24)