Environmental application of elemental speciation analysis based on liquid or gas chromatography hyphenated to inductively coupled plasma mass spectrometry-A review

被引:103
作者
Popp, Maximilian [1 ]
Hann, Stephan [1 ]
Koellensperger, Gunda [1 ]
机构
[1] Univ Nat Resources & Appl Life Sci, BOKU Vienna, Div Analyt Chem, Dept Chem, A-1190 Vienna, Austria
关键词
Elemental speciation analysis; Environmental analysis; LC-ICP-MS; GC-ICP-MS; GC-ICP-MS; SOLID-PHASE MICROEXTRACTION; ISOTOPE-DILUTION ANALYSIS; HYDROPHILIC INTERACTION CHROMATOGRAPHY; INVESTIGATE EXTRACTION PROCEDURES; SUPPRESSED ION CHROMATOGRAPHY; AGENT DEGRADATION-PRODUCTS; WASTE-WATER TREATMENT; BUTYLTIN COMPOUNDS; ARSENIC SPECIATION;
D O I
10.1016/j.aca.2010.04.036
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
In recent years the number of environmental applications of elemental speciation analysis using inductively coupled plasma mass spectrometry (ICP-MS) as detector has increased significantly. The analytical characteristics, such as extremely low detection limits (LOD) for almost all elements, the wide linear range, the possibility for multi-elemental analysis and the possibility to apply isotope dilution mass spectrometry (IDMS) make ICP-MS an attractive tool for elemental speciation analysis. Two methodological approaches, i.e. the combination of ICP-MS with high performance liquid chromatography (HPLC) and gas chromatography (GC), dominate the field. Besides the investigation of metals and metalloids and their species (e.g. Sn, Hg, As). representing "classic" elements in environmental science, more recently other elements (e.g. P, S, Br, I) amenable to ICP-MS determination were addressed. In addition, the introduction of isotope dilution analysis and the development of isotopically labeled species-specific standards have contributed to the success of ICP-MS in the field. The aim of this review is to summarize these developments and to highlight recent trends in the environmental application of ICP-MS coupled to GC and H PLC. (c) 2010 Elsevier B.V. All rights reserved.
引用
收藏
页码:114 / 129
页数:16
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