Low thermal conductivity Hf6Ta2O17 ceramics fabricated by solvothermal and pressure-less sintering

被引:31
作者
Li, Hao [1 ]
Yu, Yiping [1 ]
Wang, Song [1 ]
Xiao, Peng [1 ]
Hu, Taotao [1 ]
机构
[1] Natl Univ Def Technol, Coll Aerosp Sci & Engn, Sci & Technol Adv Ceram Fibers & Composites Lab, Changsha 410073, Hunan, Peoples R China
关键词
Solvothermal method; Pressure-less sintering; Thermophysical property; Thermal barrier coatings; HIGH-TEMPERATURE; EXPANSION; PRECURSOR;
D O I
10.1016/j.ceramint.2021.03.091
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
In the present work, single-phase Hf6Ta2O17 spherical powders with uniform particle sizes were successfully synthesized by a solvothermal method and heat treatment at a relatively low temperature (1000 degrees C). After pressure-less sintering at 1700 degrees C, bulk ceramics with a relative density of 96.30% could be obtained, and the micromorphology was combined by large rod-shaped particles. The thermophysical property of Hf6Ta2O17 ceramics and the influencing factors were investigated. The thermal conductivity was 1.62 W/(m center dot K) at 1500 degrees C, which was lower than that of traditional 8YSZ, indicating that Hf6Ta2O17 was more suitable for thermal barrier coatings. Doping other elements could be expected to improve the properties of Hf6Ta2O17 ceramics.
引用
收藏
页码:17711 / 17718
页数:8
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