Magnetic ordering in frustrated Ce5Ni2Si3 -: art. no. 224409

被引:17
作者
Lee, BK
Ryu, DH
Kim, DY
Hong, JB
Jung, MH
Kitazawa, H
Suzuki, O
Kimura, S
Kwon, YS [1 ]
机构
[1] Sungkyunkwan Univ, Phys Res Div BK21, Suwon 440746, South Korea
[2] Sungkyunkwan Univ, Inst Basic Sci, Suwon 440746, South Korea
[3] Korea Basic Sci Inst, Mat Sci Team, Taejon 305333, South Korea
[4] Natl Inst Mat Sci, Tsukuba, Ibaraki 3050047, Japan
[5] Inst Mol Sci, UVSOR Facil, Okazaki, Aichi 4448585, Japan
[6] Seoul Natl Univ, Ctr Strongly Correlated Mat Res, Seoul 151742, South Korea
关键词
D O I
10.1103/PhysRevB.70.224409
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The transport, magnetic, and thermal properties are studied on an antiferromagnetic compound Ce5Ni2Si3 with T-N=7.3 K. We find signatures of spin fluctuation in this geometrically frustrated magnet. The Curie-Weiss fit gives a large value of the paramagnetic Curie temperature, yielding a frustration parameter f=8.4. The electronic specific heat coefficient gamma=300 mJ/Ce mol K-2 is strongly enhanced, leading to residual entropy at low temperatures. The spin fluctuation is suppressed as the magnetic field exceeds the metamagnetic transition field H-m=1 T, where the magnetoresistance decreases steeply. The steady increase of magnetic susceptibility below T-N is likely to be associated with the presence of paramagnetic Ce ions. For La5Ni2Si3, a superconducting transition is observed at T-c=1.8 K.
引用
收藏
页码:224409 / 1
页数:5
相关论文
共 13 条
[1]  
Bodak O. I., 1972, Soviet Physics - Crystallography, V17, P439
[2]   EXCHANGE INTERACTION IN ALLOYS WITH CERIUM IMPURITIES [J].
COQBLIN, B ;
SCHRIEFF.JR .
PHYSICAL REVIEW, 1969, 185 (02) :847-+
[3]   COMMENSURATE-INCOMMENSURATE MAGNETIC PHASE-TRANSITIONS OF CEPTAL [J].
DONNI, A ;
KITAZAWA, H ;
FISCHER, P ;
TANG, J ;
KOHGI, M ;
ENDOH, Y ;
MORII, Y .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1995, 7 (08) :1663-1678
[4]   Low temperature spin dynamics of the geometrically frustrated antiferromagnetic garnet Gd3Ga5O12 [J].
Dunsiger, SR ;
Gardner, JS ;
Chakhalian, JA ;
Cornelius, AL ;
Jaime, M ;
Kiefl, RF ;
Movshovich, R ;
MacFarlane, WA ;
Miller, RI ;
Sonier, JE ;
Gaulin, BD .
PHYSICAL REVIEW LETTERS, 2000, 85 (16) :3504-3507
[5]   Kondo screening and magnetic ordering in frustrated UNi4B [J].
Lacroix, C ;
Canals, B ;
NunezRegueiro, MD .
PHYSICAL REVIEW LETTERS, 1996, 77 (25) :5126-5129
[6]   MAGNETIC-ORDERING AND FRUSTRATION IN HEXAGONAL UNI4B [J].
MENTINK, SAM ;
DROST, A ;
NIEUWENHUYS, GJ ;
FRIKKEE, E ;
MENOVSKY, AA ;
MYDOSH, JA .
PHYSICAL REVIEW LETTERS, 1994, 73 (07) :1031-1034
[7]   MAGNETIZATION AND RESISTIVITY OF UNI4B IN HIGH MAGNETIC-FIELDS [J].
MENTINK, SAM ;
NIEUWENHUYS, GJ ;
NAKOTTE, H ;
MENOVSKY, AA ;
DROST, A ;
FRIKKEE, E ;
MYDOSH, JA .
PHYSICAL REVIEW B, 1995, 51 (17) :11567-11573
[8]   Second low-temperature phase transition in frustrated UNi4B [J].
Movshovich, R ;
Jaime, M ;
Mentink, S ;
Menovsky, AA ;
Mydosh, JA .
PHYSICAL REVIEW LETTERS, 1999, 83 (10) :2065-2068
[9]   Preparation, crystal structure, heat capacity, magnetism, and the magnetocaloric effect of Pr5Ni1.9Si3 and PrNi -: art. no. 134452 [J].
Pecharsky, AO ;
Mozharivskyj, Y ;
Dennis, KW ;
Gschneidner, KA ;
McCallum, RW ;
Miller, GJ ;
Pecharsky, VK .
PHYSICAL REVIEW B, 2003, 68 (13)
[10]   MAGNETIC-SUSCEPTIBILITY AND SPECIFIC-HEAT OF THE COQBLIN-SCHRIEFFER MODEL [J].
RAJAN, VT .
PHYSICAL REVIEW LETTERS, 1983, 51 (04) :308-311