Preparation of ordered mesoporous Ag/WO3 and its highly efficient degradation of acetaldehyde under visible-light irradiation

被引:159
作者
Sun, Songmei [1 ]
Wang, Wenzhong [1 ]
Zeng, Shaozhong [1 ]
Shang, Meng [1 ]
Zhang, Ling [1 ]
机构
[1] Chinese Acad Sci SICCAS, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China
基金
中国国家自然科学基金;
关键词
Photocatalyst; Tungsten trioxide; Silver loaded; Mesoporous structure; ENHANCED PHOTOCATALYTIC ACTIVITY; DRIVEN PHOTOCATALYSTS; TITANIUM-DIOXIDE; TUNGSTEN-OXIDE; THIN-FILMS; TIO2; WO3; OXIDATION; NANOCOMPOSITES; RECOMBINATION;
D O I
10.1016/j.jhazmat.2010.01.098
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A highly active photocatalyst, silver loaded mesoporous WO3, was successfully synthesized by an ultrasound assisted insertion method. The photodegradation of a common air pollutant acetaldehyde was adopted to evaluate the photocatalytic performance of the as-prepared sample under visible-light irradiation. The photocatalytic activity was about three and six times higher than that of pure mesoporous WO3 and nitrogen-doped TiO2, respectively. The photocatalytic mechanism was investigated to understand the much enhanced photocatalytic activity, which was mainly attributed to the largely improved electron-hole separation in the Ag-WO3 heterojunction. (C) 2010 Elsevier B.V. All rights reserved.
引用
收藏
页码:427 / 433
页数:7
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