Highly efficient visible light driven photocatalytic activities of the LaCuS2-graphene composite-decorated ordered mesoporous silica

被引:12
作者
Dinh Cung Tien Nguyen [1 ]
Woo, Jung-Hun [1 ]
Cho, Kwang Youn [2 ]
Jung, Chong-Hun [3 ]
Oh, Won-Chun [1 ]
机构
[1] Hanseo Univ, Dept Adv Mat Sci & Engn, Seosan 356706, Chungnam, South Korea
[2] Korea Inst Ceram Engn & Technol, Jinju Si, Gyeongsangnam D, South Korea
[3] Korean Atom Energy Res Inst, Decontaminat & Decommissing Res Div, POB 105, Yuseong 305600, Daejeon, South Korea
关键词
Graphene-based nanocomposite; LaCuS2; nanoparticles; Mesoporous silica; Dye decomposition; Gallic acid degradation; Hydrogen production; GRAPHENE; NANOCOMPOSITES; ADSORPTION; CUO; FABRICATION; SURFACTANT; MORPHOLOGY;
D O I
10.1016/j.seppur.2018.05.019
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
A combination of mesoporous silica with an LaCuS2-graphene composite has been prepared by a self-assembly method in support of the CTAB surfactant as the structure creator and basic medium. The characterization was investigated using XRD, SEM, TEM, HR-TEM, EDS, XPS, Raman, and DRS analysis. The pore size of the as-fabricated composite was calculated to be 5.83 nm by the nitrogen adsorption/desorption isotherms. In addition, the photocatalytic properties revealed that the mesoporous SiO2/LaCuS2-graphene catalyst presented a good result for the photocatalytic activity of organic dyes and gallic acid under visible light irradiation. Moreover, the as-prepared mesoporous SiO2/LaCuS2-graphene nanocomposite exhibited a good photodegradation rate for a cationic organic dye group under a pH medium of 11. The photocatalytic performance of the phenol compound representation presented a good result, and the optimum amount of the catalytic for the gallic acid photocatalytic activity is 0.05 g. In addition, the mesoporous SiO2/LaCuS2-graphene catalyst can be exploited for the application of solar energy conversion with high hydrogen production capacity.
引用
收藏
页码:11 / 21
页数:11
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