Investigating two-photon double ionization of D2 by XUV-pump-XUV-probe experiments

被引:49
|
作者
Jiang, Y. H. [1 ]
Rudenko, A. [2 ]
Perez-Torres, J. F. [3 ]
Herrwerth, O. [4 ]
Foucar, L. [2 ]
Kurka, M. [1 ]
Kuehnel, K. U. [1 ]
Toppin, M. [1 ]
Plesiat, E. [3 ]
Morales, F. [3 ]
Martin, F. [3 ]
Lezius, M. [4 ]
Kling, M. F. [4 ]
Jahnke, T. [5 ]
Doerner, R. [5 ]
Sanz-Vicario, J. L. [6 ]
van Tilborg, J. [7 ]
Belkacem, A. [7 ]
Schulz, M. [8 ]
Ueda, K. [9 ]
Zouros, T. J. M. [10 ]
Duesterer, S. [11 ]
Treusch, R. [11 ]
Schroeter, C. D. [1 ]
Moshammer, R. [1 ]
Ullrich, J. [1 ,2 ]
机构
[1] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany
[2] CFEL, Max Planck Adv Study Grp, D-22607 Hamburg, Germany
[3] Univ Autonoma Madrid, Dept Quim C9, E-28049 Madrid, Spain
[4] Max Planck Inst Quantum Opt, D-85748 Garching, Germany
[5] Goethe Univ Frankfurt, Inst Kernphys, D-60486 Frankfurt, Germany
[6] Univ Antioquia, Inst Fis, Medellin, Colombia
[7] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA
[8] Missouri Univ Sci & Technol Rolla, Rolla, MO 65409 USA
[9] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Sendai, Miyagi 9808577, Japan
[10] Univ Crete, Dept Phys, Iraklion 71003, Crete, Greece
[11] DESY, D-22607 Hamburg, Germany
来源
PHYSICAL REVIEW A | 2010年 / 81卷 / 05期
基金
美国国家科学基金会;
关键词
FREE-ELECTRON LASER; EXTREME-ULTRAVIOLET; COHERENCE; DYNAMICS;
D O I
10.1103/PhysRevA.81.051402
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We used a split-mirror setup attached to a reaction microscope at the free-electron laser in Hamburg (FLASH) to perform an XUV-pump-XUV-probe experiment by tracing the ultrafast nuclear wave-packet motion in the D-2(+)(1s sigma(g)) with 10 fs time resolution. Comparison with time-dependent calculations shows excellent agreement with the measured vibrational period of 22 +/- 4 fs in D-2(+), points to the importance of accurately knowing the internuclear distance-dependent ionization probability, and paves the way to control sequential and nonsequential two-photon double-ionization contributions.
引用
收藏
页数:4
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