Graphdiyne-based photocatalysts for solar fuel production

被引：51

作者：

Bie, Chuanbiao ^{[1
]}

Cheng, Bei ^{[2
]}

Ho, Wingkei ^{[3
]}

Li, Youji ^{[4
]}

Macyk, Wojciech ^{[5
]}

Ghasemi, Jahan B. ^{[6
]}

Yu, Jiaguo ^{[1
]}

机构：

[1] China Univ Geosci, Fac Mat Sci & Chem, Lab Solar Fuel, 388 Lumo Rd, Wuhan 430074, Peoples R China

[2] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China

[3] Educ Univ Hong Kong, Dept Sci & Environm Studies, Tai Po, Hong Kong 999077, Peoples R China

[4] Jishou Univ, Coll Chem & Chem Engn, Jishou 416000, Hunan, Peoples R China

[5] Jagiellonian Univ, Fac Chem, Ul Gronostajowa 2, PL-30387 Krakow, Poland

[6] Univ Tehran, Sch Sci, Fac Chem, Tehran, Iran

来源：

GREEN CHEMISTRY | 2022年 / 24卷 / 15期

基金：

中国国家自然科学基金; 中国博士后科学基金;

关键词：

CO2; REDUCTION; ELECTRONIC-PROPERTIES; HYDROGEN GENERATION; CARRIER MOBILITY; CARBON; GRAPHYNE; GRAPHENE; NITROGEN; SURFACE; WATER;

D O I：

10.1039/d2gc01684b

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Graphdiyne is an emerging material widely used in photocatalysis. Its excellent physicochemical properties, such as nonuniform electron distribution, uniform pore distribution, excellent electron mobility, and high chemical stability, make it promising for solar fuel production. Given the rapid development of graphdiyne-based photocatalysts and their application in solar fuel production, a timely review of this field is urgently needed. This paper summarises the structure, properties, synthesis and characterisation of graphdiyne, and the achievements of graphdiyne-based photocatalysts in solar fuel production, including H-2 evolution, CO2 reduction and N-2 fixation. The challenges and outlook of graphdiyne-based photocatalysts for efficient solar fuel production are presented. This paper is expected to provide new insights into graphdiyne-based photocatalysts for solar fuel production.

引用

页码：5739 / 5754

页数：16

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