Stable metal-organic frameworks for PEC water splitting

被引：17
作者：
Gong, Yun-Nan [1 ,2 ]
Liu, Jin-Wang [2 ]
Shao, Bi-Zhu [2 ]
Zhong, Di-Chang [1 ]
Lu, Tong-Bu [1 ]
机构：
[1] Tianjin Univ Technol, Sch Mat Sci & Engn, Sch Chem & Chem Engn, Inst New Energy Mat & Low Carbon Technol, Tianjin 300384, Peoples R China
[2] Gannan Normal Univ, Key Lab Jiangxi Univ Funct Mat Chem, Coll Chem & Chem Engn, Ganzhou 341000, Jiangxi, Peoples R China
来源：
FLATCHEM | 2021年 / 27卷
基金：
中国国家自然科学基金;
关键词：
Metal-organic frameworks; Stability; Photoelectrocatalysts; Water splitting; PORE-SIZE; SELECTIVE ADSORPTION; STABILITY; MOF; CONVERSION; FACILE; GAS; PHOTOANODE; NANOSHEETS; CAPTURE;
D O I：
10.1016/j.flatc.2021.100240
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Photoelectrochemical (PEC) water splitting into H2 and O2 has been regarded as a promising strategy to achieve solar-to-chemical energy conversion. Metal-organic frameworks (MOFs) are emerging as promising photoelectrocatalysts for this significant energy conversion reaction owing to their unique photochemical and textural properties. In this review, we summarized recent advances in the construction of stable MOFs for PEC water splitting, involving main group metal-carboxylate frameworks, transition metal-carboxylate frameworks, transition metal-azolate frameworks, rare earth metal-carboxylate frameworks, as well as post-synthetic MOFs. We particularly analyzed and discussed the correlation between catalytic performance and catalyst structures, based on which, we put forward a perspective for construction of efficient MOFs for PEC water splitting.
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页数：10
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