Nanocellulose-Assisted Thermally Induced Growth of Silver Nanoparticles for Optical Applications

被引：16

作者：

Brett, Calvin J. ^{[1
,2
,7
]}

Ohm, Wiebke ^{[1
]}

Fricke, Bjorn ^{[1
]}

Alexakis, Alexandros E. ^{[2
,3
]}

Laarmann, Tim ^{[1
,4
]}

Korstgens, Volker ^{[5
]}

Muller-Buschbaum, Peter ^{[5
,6
]}

Soderberg, L. Daniel ^{[2
,7
]}

Roth, Stephan, V ^{[1
,3
]}

机构：

[1] Forschungszentrum Helmholtz Gemeinschaft, Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany

[2] KTH Royal Inst Technol, Wallenberg Wood Sci Ctr, S-10044 Stockholm, Sweden

[3] Dept Fibre & Polymer Technol, Div Coating Technol, S-10044 Stockholm, Sweden

[4] Hamburg Ctr Ultrafast Imaging CUI, D-22761 Hamburg, Germany

[5] Tech Univ Munich, Phys Dept, Lehrstuhl Funkt Materialien, D-85748 Garching, Germany

[6] Tech Univ Munich, Heinz Maier Leibnitz Zentrum MLZ, D-85748 Garching, Germany

[7] KTH Royal Inst Technol, Dept Engn Mech, S-10044 Stockholm, Sweden

来源：

ACS APPLIED MATERIALS & INTERFACES | 2021年 / 13卷 / 23期

关键词：

cellulose; silver plasmonics; X-ray scattering; thin films; nucleation and growth; nanoparticles; MORPHOLOGICAL PROPERTIES; CELLULOSE NANOPAPER; SPRAY; EFFICIENCY;

D O I：

10.1021/acsami.1c07544

中图分类号：

TB3 [工程材料学];

学科分类号：

0805 ; 080502 ;

摘要：

Optically responsive materials are present in everyday life, from screens to sensors. However, fabricating large-area, fossil-free materials for functional biocompatible applications is still a challenge today. Nanocelluloses from various sources, such as wood, can provide biocompatibility and are emerging candidates for templating organic optoelectronics. Silver (Ag) in its nanoscale form shows excellent optical properties. Herein, we combine both materials using thin-film large-area spray-coating to study the fabrication of optical response applications. We characterize the Ag nanoparticle formation by X-ray scattering and UV-vis spectroscopy in situ during growth on the nanocellulose template. The morphology and optical properties of the nanocellulose film are compared to the rigid reference surface SiO2. Our results clearly show the potential to tailor the energy band gap of the resulting hybrid material.

引用

页码：27696 / 27704

页数：9

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