Efficient fuel utilization by enhancing the under-rib mass transport using new serpentine flow field designs of direct methanol fuel cells

被引:52
作者
El-Zoheiry, Radwan M. [1 ]
Ookawara, Shinichi [1 ,2 ]
Ahmed, Mahmoud [1 ]
机构
[1] Egypt Japan Univ Sci & Technol, Dept Energy Resources Engn, New Borg El Arab, Egypt
[2] Tokyo Inst Technol, Dept Chem Sci & Engn, Tokyo 1528552, Japan
关键词
Direct methanol fuel cells; Under-rib flow; Serpentine flow field; GAS-DIFFUSION LAYER; COMPUTATIONAL SIMULATION; LIMITING CURRENT; PERFORMANCE; ANODE; 2-PHASE; CHANNEL; CONVECTION; MODEL; ENHANCEMENT;
D O I
10.1016/j.enconman.2017.04.041
中图分类号
O414.1 [热力学];
学科分类号
摘要
New serpentine flow field designs of direct methanol fuel cells have been developed to enhance the under rib reactant mass transport without affecting the electronic conductivity to boost up the fuel utilization and fuel cell efficiency. The flow field design is based on three main criteria including the number of paths, the rib lengths, and the flow-path patterning in channels. Therefore, six different flow field designs are developed, including one design with two paths, two designs with three paths and different patterning and rib lengths, and three designs with four paths, different patterning and rib lengths. A three-dimensional single phase model for the direct methanol fuel cell is developed, simulated numerically and validated using the available experimental data. Results revealed that a significant enhancement of fuel cell performance is attained using the new designs. The design with the longest ribs and four paths attains the highest under-rib flows, and the lowest pressure drop between inlet and outlet. Furthermore, the power density has shown a 52.9% and 35.8% increase using an enhanced serpentine flow field with four paths compared to the conventional serpentine flow field design, at 0.5 M and 0.25 M inlet methanol concentrations. Using the new designs allows for the operating of the direct methanol fuel cell at a lower methanol concentration without a significant reduction of the output power. (C) 2017 Elsevier Ltd. All rights reserved.
引用
收藏
页码:88 / 103
页数:16
相关论文
共 43 条
[1]   A review on methanol crossover in direct methanol fuel cells: challenges and achievements [J].
Ahmed, Mahmoud ;
Dincer, Ibrahim .
INTERNATIONAL JOURNAL OF ENERGY RESEARCH, 2011, 35 (14) :1213-1228
[2]   Modeling optimizes PEM fuel cell performance using three-dimensional multi-phase computational fluid dynamics model [J].
Al-Baghdadi, Maher A. R. Sadiq ;
Al-Janabi, Haroun A. K. Shahad .
ENERGY CONVERSION AND MANAGEMENT, 2007, 48 (12) :3102-3119
[3]   Nature inspired flow field designs for proton exchange membrane fuel cell [J].
Arvay, A. ;
French, J. ;
Wang, J. -C. ;
Peng, X. -H. ;
Kannan, A. M. .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2013, 38 (09) :3717-3726
[4]   A numerical study on the performance of polymer electrolyte membrane fuel cells due to the variation in gas diffusion layer permeability [J].
Baek, Seung Man ;
Koh, Soo Gon ;
Kim, Kwang Nam ;
Kang, Jung Ho ;
Nam, Jin Hyun ;
Kim, Charn-Jung .
JOURNAL OF MECHANICAL SCIENCE AND TECHNOLOGY, 2011, 25 (02) :457-467
[5]   Review and advances of direct methanol fuel cells: Part II: Modeling and numerical simulation [J].
Bahrami, Hafez ;
Faghri, Amir .
JOURNAL OF POWER SOURCES, 2013, 230 :303-320
[6]   Water Management in a Passive DMFC Using Highly Concentrated Methanol Solution [J].
Bahrami, Hafez ;
Faghri, Amir .
JOURNAL OF FUEL CELL SCIENCE AND TECHNOLOGY, 2011, 8 (02)
[7]   A symmetrical, planar SOFC design for NASN′s high specific power density requirements [J].
Cable, Thomas L. ;
Sofie, Stephen W. .
JOURNAL OF POWER SOURCES, 2007, 174 (01) :221-227
[8]   Current Advances in Polymer Electrolyte Fuel Cells Based on the Promotional Role of Under-rib Convection [J].
Choi, K. -S. ;
Kim, B. -G. ;
Park, K. ;
Kim, H. -M. .
FUEL CELLS, 2012, 12 (06) :908-938
[9]   Flow control of under-rib convection enhancing the performance of proton exchange membrane fuel cell [J].
Choi, Kap-Seung ;
Kim, Beom-Gi ;
Park, Kiwon ;
Kim, Hyung-Man .
COMPUTERS & FLUIDS, 2012, 69 :81-92
[10]   On the relative influence of convection in serpentine flow fields of PEM fuel cells [J].
Feser, J. P. ;
Prasad, A. K. ;
Advani, S. G. .
JOURNAL OF POWER SOURCES, 2006, 161 (01) :404-412