Effects of surface plasmon polariton-mediated interactions on second harmonic generation from assemblies of pyramidal metallic nano-cavities

被引：20

作者：

Kolkowski, Radoslaw ^{[1
,2
]}

Szeszko, Justyna ^{[3
]}

Dwir, Benjamin ^{[3
]}

Kapon, Eli ^{[3
]}

Zyss, Joseph ^{[1
]}

机构：

[1] Ecole Normale Super, Lab Photon Quant & Mol, F-94230 Cachan, France

[2] Wroclaw Univ Technol, Inst Phys & Theoret Chem, PL-50370 Wroclaw, Poland

[3] Swiss Fed Inst Technol Lausanne EPFL, Lab Phys Nanostruct, CH-1015 Lausanne, Switzerland

来源：

OPTICS EXPRESS | 2014年 / 22卷 / 25期

基金：

瑞士国家科学基金会;

关键词：

GOLD NANOPARTICLES; NANOAPERTURES; ENHANCEMENT; MOLECULES; ANTENNAS; ARRAYS;

D O I：

10.1364/OE.22.030592

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

We use polarization-resolved two-photon microscopy to investigate second harmonic generation (SHG) from individual assemblies of site-controlled nano-pyramidal recess templates covered with silver films. We demonstrate the effect of the surface plasmon polaritons (SPPs) at fundamental and second-harmonic frequencies on the effective second order susceptibility tensor as a function of pyramid arrangement and inter-pyramid distance. These results open new perspectives for the application of SHG microscopy as a sensitive probe of coherently excited SPPs, as well as for the design of new plasmonic nanostructure assemblies with tailored nonlinear optical properties. (C)2014 Optical Society of America

引用

页码：30592 / 30606

页数：15

共 7 条

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