The Improvement of Photocatalysis H2 Evolution Over g-C3N4 With Na and Cyano-Group Co-modification

被引:33
|
作者
Liu, Gang [1 ]
Yan, Song [1 ]
Shi, Lei [1 ]
Yao, Lizhu [1 ]
机构
[1] Liaoning Shihua Univ, Coll Chem Chem Engn & Environm Engn, Fushun, Peoples R China
来源
FRONTIERS IN CHEMISTRY | 2019年 / 7卷
关键词
graphitic carbon nitride; Na and cyano-group co-modification; photocatalysis; H-2; evolution; sustainable; GRAPHITIC CARBON NITRIDE; NITROGEN-VACANCY; DOPED G-C3N4; WATER; DEGRADATION; SEMICONDUCTORS; SURFACE; SITES; FUELS;
D O I
10.3389/fchem.2019.00639
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Na and cyano-group co-modified g-C3N4 was easily synthesized and its physicochemical property was completely analyzed. The results manifested that Na and cyano-group modification could heighten visible light absorbed ability and accelerate photoinduced charge separation. When resultant Na and cyano-group co-modified g-C3N4 was splitting water H-2 evolution, its H-2 evolution rate was obviously improved. Furthermore, it also kept excellent stable capacity of H-2 evolution and stability of chemical structure. Hence, this present study does not only develop an efficient strategy to boost photocatalytic property of g-C3N4 based catalysts, but also provides useful guidance for designing more effective photocatalysts.
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页数:7
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