Following the dynamics of matter with femtosecond precision using the X-ray streaking method

被引：25

作者：

David, C. ^{[1
]}

Karvinen, P. ^{[1
]}

Sikorski, M. ^{[2
]}

Song, S. ^{[2
]}

Vartiainen, I. ^{[1
]}

Milne, C. J. ^{[1
]}

Mozzanica, A. ^{[1
]}

Kayser, Y. ^{[1
]}

Diaz, A. ^{[1
]}

Mohacsi, I. ^{[1
]}

Carini, G. A. ^{[2
]}

Herrmann, S. ^{[2
]}

Farm, E. ^{[3
]}

Ritala, M. ^{[3
]}

Fritz, D. M. ^{[2
]}

Robert, A. ^{[2
]}

机构：

[1] Paul Scherrer Inst, CH-5232 Villigen, Switzerland

[2] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA

[3] Univ Helsinki, Dept Chem, FI-00014 Helsinki, Finland

来源：

SCIENTIFIC REPORTS | 2015年 / 5卷

关键词：

FREE-ELECTRON LASER; PUMP-PROBE EXPERIMENTS; EXTREME-ULTRAVIOLET; DELAY-LINE; GENERATION; OPERATION; PULSES;

D O I：

10.1038/srep07644

中图分类号：

O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];

学科分类号：

07 ; 0710 ; 09 ;

摘要：

X-ray Free Electron Lasers (FELs) can produce extremely intense and very short pulses, down to below 10 femtoseconds (fs). Among the key applications are ultrafast time-resolved studies of dynamics of matter by observing responses to fast excitation pulses in a pump-probe manner. Detectors with sufficient time resolution for observing these processes are not available. Therefore, such experiments typically measure a sample's full dynamics by repeating multiple pump-probe cycles at different delay times. This conventional method assumes that the sample returns to an identical or very similar state after each cycle. Here we describe a novel approach that can provide a time trace of responses following a single excitation pulse, jitter-free, with fs timing precision. We demonstrate, in an X-ray diffraction experiment, how it can be applied to the investigation of ultrafast irreversible processes.

引用

页数：6

共 30 条

[1] Atomic layer deposition of iridium thin films [J].

Aaltonen, T ;

Ritala, M ;

Sammelselg, V ;

Leskelä, M .

JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2004, 151 (08) :G489-G492

[2] Operation of a free-electron laser from the extreme ultraviolet to the water window [J].

Ackermann, W. ;

Asova, G. ;

Ayvazyan, V. ;

Azima, A. ;

Baboi, N. ;

Baehr, J. ;

Balandin, V. ;

Beutner, B. ;

Brandt, A. ;

Bolzmann, A. ;

Brinkmann, R. ;

Brovko, O. I. ;

Castellano, M. ;

Castro, P. ;

Catani, L. ;

Chiadroni, E. ;

Choroba, S. ;

Cianchi, A. ;

Costello, J. T. ;

Cubaynes, D. ;

Dardis, J. ;

Decking, W. ;

Delsim-Hashemi, H. ;

Delserieys, A. ;

Di Pirro, G. ;

Dohlus, M. ;

Duesterer, S. ;

Eckhardt, A. ;

Edwards, H. T. ;

Faatz, B. ;

Feldhaus, J. ;

Floettmann, K. ;

Frisch, J. ;

Froehlich, L. ;

Garvey, T. ;

Gensch, U. ;

Gerth, Ch. ;

Goerler, M. ;

Golubeva, N. ;

Grabosch, H.-J. ;

Grecki, M. ;

Grimm, O. ;

Hacker, K. ;

Hahn, U. ;

Han, J. H. ;

Honkavaara, K. ;

Hott, T. ;

Huening, M. ;

Ivanisenko, Y. ;

Jaeschke, E. .

NATURE PHOTONICS, 2007, 1 (06) :336-342

[3]

Barty A, 2012, NAT PHOTONICS, V6, P35, DOI [10.1038/NPHOTON.2011.297, 10.1038/nphoton.2011.297]

[4] Femtosecond XANES Study of the Light-Induced Spin Crossover Dynamics in an Iron(II) Complex [J].

Bressler, Ch. ;

Milne, C. ;

Pham, V. -T. ;

ElNahhas, A. ;

van der Veen, R. M. ;

Gawelda, W. ;

Johnson, S. ;

Beaud, P. ;

Grolimund, D. ;

Kaiser, M. ;

Borca, C. N. ;

Ingold, G. ;

Abela, R. ;

Chergui, M. .

SCIENCE, 2009, 323 (5913) :489-492

[5] X-ray split and delay system for soft x-ray at LCLS [J].

Castagna, J. C. ;

Murphy, B. ;

Bozek, J. ;

Berrah, N. .

11TH INTERNATIONAL CONFERENCE ON SYNCHROTRON RADIATION INSTRUMENTATION (SRI 2012), 2013, 425

[6] Femtosecond X-ray protein nanocrystallography [J].

Chapman, Henry N. ;

Fromme, Petra ;

Barty, Anton ;

White, Thomas A. ;

Kirian, Richard A. ;

Aquila, Andrew ;

Hunter, Mark S. ;

Schulz, Joachim ;

DePonte, Daniel P. ;

Weierstall, Uwe ;

Doak, R. Bruce ;

Maia, Filipe R. N. C. ;

Martin, Andrew V. ;

Schlichting, Ilme ;

Lomb, Lukas ;

Coppola, Nicola ;

Shoeman, Robert L. ;

Epp, Sascha W. ;

Hartmann, Robert ;

Rolles, Daniel ;

Rudenko, Artem ;

Foucar, Lutz ;

Kimmel, Nils ;

Weidenspointner, Georg ;

Holl, Peter ;

Liang, Mengning ;

Barthelmess, Miriam ;

Caleman, Carl ;

Boutet, Sebastien ;

Bogan, Michael J. ;

Krzywinski, Jacek ;

Bostedt, Christoph ;

Bajt, Sasa ;

Gumprecht, Lars ;

Rudek, Benedikt ;

Erk, Benjamin ;

Schmidt, Carlo ;

Hoemke, Andre ;

Reich, Christian ;

Pietschner, Daniel ;

Strueder, Lothar ;

Hauser, Guenter ;

Gorke, Hubert ;

Ullrich, Joachim ;

Herrmann, Sven ;

Schaller, Gerhard ;

Schopper, Florian ;

Soltau, Heike ;

Kuehnel, Kai-Uwe ;

Messerschmidt, Marc .

NATURE, 2011, 470 (7332) :73-U81

[7] Nanofocusing of hard X-ray free electron laser pulses using diamond based Fresnel zone plates [J].

David, C. ;

Gorelick, S. ;

Rutishauser, S. ;

Krzywinski, J. ;

Vila-Comamala, J. ;

Guzenko, V. A. ;

Bunk, O. ;

Farm, E. ;

Ritala, M. ;

Cammarata, M. ;

Fritz, D. M. ;

Barrett, R. ;

Samoylova, L. ;

Gruenert, J. ;

Sinn, H. .

SCIENTIFIC REPORTS, 2011, 1

[8] Wavelength tunable diffractive transmission lens for hard x rays [J].

David, C ;

Nöhammer, B ;

Ziegler, E .

APPLIED PHYSICS LETTERS, 2001, 79 (08) :1088-1090

[9] Photoinduced structural dynamics of polar solids studied by femtosecond X-ray diffraction [J].

Elsaesser, Thomas ;

Woerner, Michael .

ACTA CRYSTALLOGRAPHICA SECTION A, 2010, 66 :168-178

[10]

Emma P, 2010, NAT PHOTONICS, V4, P641, DOI [10.1038/nphoton.2010.176, 10.1038/NPHOTON.2010.176]

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