Expanding light utilization to the near-infrared region for hybrid bio-photoelectrochemical cells

被引：2

作者：

Zhang, Lingling ^{[1
]}

Zhang, He ^{[1
,2
]}

Zhang, Xiaowei ^{[1
,2
]}

Han, Yujie ^{[1
,2
]}

Zhang, Hui ^{[1
,2
]}

Zhai, Yiwen ^{[1
,2
]}

Dong, Shaojun ^{[1
,2
]}

机构：

[1] Chinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Jilin, Peoples R China

[2] Univ Chinese Acad Sci, Beijing 100049, Peoples R China

来源：

NANOSCALE | 2017年 / 9卷 / 27期

基金：

中国国家自然科学基金;

关键词：

UP-CONVERSION NANOPARTICLES; SOLAR-CELLS; CONVERTING PHOSPHORS; HIGHLY UNIFORM; PERFORMANCE; PHOTOCATALYSIS; LUMINESCENCE; HYDROGEN;

D O I：

10.1039/c7nr02636f

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The insatiable energy demand asks for the maximum conversion of green renewable sources. Herein, we propose the first NIR-assisted glucose/air bio-photoelectrochemical (BPEC) cell comprising a rare earth up-conversion microcrystal (UCMC)-based polyterthiophene (pTTh) cathode. Upon irradiation with a 980 nm laser, UCMCs emit robust luminescence in the visible range, which can efficiently excite pTTh, catalyzing the reduction of oxygen and generating photocurrent. Coupling with a glucose oxidation bioanode, this assembled BPEC cell exhibits a maximal output power density of 40.6 mu W cm(-2) and an open circuit voltage of 0.53 V. This success is an essential conceptual steppingstone towards the comprehensive utilization of whole sunlight and offers alternative solutions for multiple energy conversions.

引用

页码：9404 / 9410

页数：7

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