Source characterization of urban particles from meat smoking activities in Chongqing, China using single particle aerosol mass spectrometry

被引:42
作者
Chen, Yang [1 ,4 ]
Wenger, John C. [2 ,3 ]
Yang, Fumo [1 ,5 ,6 ]
Cao, Junji [4 ]
Huang, Rujin [4 ]
Shi, Guangming [1 ]
Zhang, Shumin [7 ,8 ]
Tian, Mi [1 ]
Wang, Huanbo [1 ]
机构
[1] Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Res Ctr Atmospher Environm, Chongqing 400714, Peoples R China
[2] Univ Coll Cork, Dept Chem, Cork, Ireland
[3] Univ Coll Cork, Environm Res Inst, Cork, Ireland
[4] Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian 710061, Peoples R China
[5] Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China
[6] Yangtze Normal Univ, Chongqing 408100, Peoples R China
[7] North Sichuan Med Coll, Nanchong 637000, Sichuan, Peoples R China
[8] Chongqing Univ, Chongqing 400044, Peoples R China
关键词
Biomass burning; Meat smoking; Chongqing; SPAMS; PM2.5; Biofuel smoldering; BIOMASS-BURNING AEROSOLS; CHEMICAL MIXING STATE; YANGTZE-RIVER DELTA; INDIVIDUAL PARTICLES; ORGANIC AEROSOLS; HAZE EVENTS; EVOLUTION; EMISSIONS; PM2.5; SIZE;
D O I
10.1016/j.envpol.2017.05.022
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A Single Particle Aerosol Mass Spectrometer (SPAMS) was deployed in the urban area of Chongqing to characterize the particles present during a severe particulate pollution event that occurred in winter 2014-2015. The measurements were made at a time when residents engaged in traditional outdoor meat smoking activities to preserve meat before the Chinese Spring Festival. The measurement period was predominantly characterized by stagnant weather conditions, highly elevated levels of PM2.5, and low visibility. Eleven major single particle types were identified, with over 92.5% of the particles attributed to biomass burning emissions. Most of the particle types showed appreciable signs of aging in the stagnant air conditions. To simulate the meat smoking activities, a series of controlled smoldering experiments was conducted using freshly cut pine and cypress branches, both with and without wood logs. SPAMS data obtained from these experiments revealed a number of biomass burning particle types, including an elemental and organic carbon (ECOC) type that proved to be the most suitable marker for meat smoking activities. The traditional activity of making preserved meat in southwestern China is shown here to be a major source of particulate pollution. Improved measures to reduce emissions from the smoking of meat should be introduced to improve air quality in regions where smoking meat activity prevails. (C) 2017 Elsevier Ltd. All rights reserved.
引用
收藏
页码:92 / 101
页数:10
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