Reforming of methane to syngas in a microwave plasma torch at atmospheric pressure

被引:68
|
作者
Chun, Se Min [1 ]
Hong, Yong Cheol [1 ,2 ]
Choi, Dae Hyun [1 ]
机构
[1] Natl Fus Res Inst, Plasma Technol Res Ctr, 37 Dongjansan Ro, Gunsan 54004, Jeollabuk Do, South Korea
[2] NPAC, 169-148 Gwahak Ro, Daejeon 305806, South Korea
关键词
Methane reforming; Microwave plasma; Synthesis gas; Syngas; HYDROGEN-PRODUCTION; CO2; CAPTURE; CATALYSTS; HYDROCARBONS; TECHNOLOGIES;
D O I
10.1016/j.jcou.2017.03.016
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Carbon dioxide was converted to synthesis gas (syngas) in a microwave plasma torch by methane reforming at atmospheric pressure. The microwave plasma torch converts CO2+CH4 into synthesis gas. This study examined conversion rates as a function of gas temperature for dry methane reforming. The temperature of the torch flame is measured 6760 K by making use of optical spectroscopy. The CO2/CH4 reforming can be completely converted into synthesis gas (conversions: 68.4%, CO2; 96.8%, CH4) through their reforming reactions at a microwave power of 6 kW. When the reforming gas (CO2:CH4) mole ratio was 1:1, the resulting synthesis gas (H-2:CO) mole ratio was 0.9:1.1. The H-2 and CO mass yield rates increased to 0.24 kg/h and 1.86 kg/h, respectively. Also, the energy yield are 240 g/h and 41.4 g/kWh. The CO2 microwave plasma torch not only exhibited noteworthy results for CO2 reduction and syngas production, but the H-2:CO mole ratio of the gas produced is easily controlled by adjusting the CO2:CH4 ratio during the feeding process. (C) 2017 Elsevier Ltd. All rights reserved.
引用
收藏
页码:221 / 229
页数:9
相关论文
共 50 条
  • [41] Study of graphene layer growth on dielectric substrate in microwave plasma torch at atmospheric pressure
    Jasek, Ondrej
    Toman, Jozef
    Jurmanova, Jana
    Snirer, Miroslav
    Kudrle, Vit
    Bursikova, Vilma
    DIAMOND AND RELATED MATERIALS, 2020, 105
  • [42] Efficient recovery of syngas from dry methane reforming product by a dual pressure swing adsorption process
    Delgado Dobladez, Jose Antonio
    Agueda Mate, Vicente Ismael
    Alvarez Torrellas, Silvia
    Larriba, Marcos
    Brea, Pablo
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2021, 46 (33) : 17522 - 17533
  • [43] Microwave Heating-Assisted Catalytic Dry Reforming of Methane to Syngas
    Hamzehlouia, Sepehr
    Jaffer, Shaffiq A.
    Chaouki, Jamal
    SCIENTIFIC REPORTS, 2018, 8
  • [44] Microwave-assisted dry reforming of methane for syngas production: a review
    T. T. Phuong Pham
    Kyoung S. Ro
    Lyufei Chen
    Devinder Mahajan
    Tan Ji Siang
    U. P. M. Ashik
    Jun-ichiro Hayashi
    Doan Pham Minh
    Dai-Viet N. Vo
    Environmental Chemistry Letters, 2020, 18 : 1987 - 2019
  • [45] Hydrogen Production via Synthetic Biogas Reforming in Atmospheric-Pressure Microwave (915MHz) Plasma at High Gas-Flow Output
    Hrycak, B.
    Czylkowski, D.
    Jasinski, M.
    Dors, M.
    Mizeraczyk, J.
    PLASMA CHEMISTRY AND PLASMA PROCESSING, 2019, 39 (03) : 695 - 711
  • [46] Syngas production from gasification of brown coal in a microwave torch plasma
    Hong, Yong C.
    Lee, Sang J.
    Shin, Dong H.
    Kim, Ye J.
    Lee, Bong J.
    Cho, Seong Y.
    Chang, Han S.
    ENERGY, 2012, 47 (01) : 36 - 40
  • [47] Hydrogen Separation from Products of Methane Reforming Reaction Carried Out in a Plasma Membrane Reactor at Low Temperature and Atmospheric Pressure
    Nguyen, Thu H.
    Mori, Shinsuke
    Suzuki, Masaaki
    JOURNAL OF CHEMICAL ENGINEERING OF JAPAN, 2010, 43 (01) : 76 - 81
  • [48] Zeolite and clay based catalysts for CO2 reforming of methane to syngas: A review
    Hambali, Hambali Umar
    Jalil, Aishah Abdul
    Abdulrasheed, Abdulrahman A.
    Siang, Tan Ji
    Gambo, Yahya
    Umar, Ahmad Abulfathi
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2022, 47 (72) : 30759 - 30787
  • [49] Plasma steam methane reforming (PSMR) using a microwave torch for commercial-scale distributed hydrogen production
    Akande, Olugbenga
    Lee, BongJu
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2022, 47 (05) : 2874 - 2884
  • [50] Microwave catalytic dry reforming of methane over Ni/SiC catalysts for efficient syngas production
    Shi, Yu
    Tian, Xiaoyan
    Deng, Zhiyong
    Wang, Fagen
    FUEL, 2025, 388