Magnetic ordering and dynamics in the XY pyrochlore antiferromagnet:: a muon-spin relaxation study of Er2Ti2O7 and Er2Sn2O7

被引:60
作者
Lago, J
Lancaster, T
Blundell, SJ
Bramwell, ST
Pratt, FL
Shirai, M
Baines, C
机构
[1] UCL, Dept Chem, London WC1H 0AJ, England
[2] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England
[3] Rutherford Appleton Lab, ISIS, Didcot OX11 0QX, Oxon, England
[4] Paul Scherrer Inst, Lab Muon Spin Spect, CH-5232 Villigen, Switzerland
关键词
D O I
10.1088/0953-8984/17/6/015
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
Spin dynamics in Er2Ti2O7 and Er2Sn2O7 have been probed by means of muon-spin relaxation (mu(+)SR) in the temperature range 0.02 less than or equal to T less than or equal to 300 K. Both compounds are thought to constitute experimental realizations of the highly frustrated XY antiferromagnet on the pyrochlore lattice, for which theory predicts fluctuation-induced magnetic order. Our results for Er2Ti2O7 are consistent with a transition into an ordered state at T-N similar to 1.1 K, in agreement with previous neutron measurements. Below this temperature, the muon relaxation rate lambda(T) remains large (similar to2 MHz) and temperature independent, in contrast to the behaviour in conventional magnets. The thermal evolution of lambda(T) for Er2Sn2O7 is somewhat similar to that of the Ti material. However, the depolarization curves remain exponential over the entire temperature range, suggesting a dense distribution of rapidly fluctuating magnetic moments, and, thus, are compatible with the absence of long-range order at least for T > 0.02 K.
引用
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页码:979 / 988
页数:10
相关论文
共 23 条
[1]  
BLOTE HWI, 1969, PHYSICA, V46, P549
[2]   Spin-polarized muons in condensed matter physics [J].
Blundell, SJ .
CONTEMPORARY PHYSICS, 1999, 40 (03) :175-192
[3]   Spin ice state in frustrated magnetic pyrochlore materials [J].
Bramwell, ST ;
Gingras, MJP .
SCIENCE, 2001, 294 (5546) :1495-1501
[4]   ORDER BY DISORDER IN AN ANISOTROPIC PYROCHLORE LATTICE ANTIFERROMAGNET [J].
BRAMWELL, ST ;
GINGRAS, MJP ;
REIMERS, JN .
JOURNAL OF APPLIED PHYSICS, 1994, 75 (10) :5523-5525
[5]  
Carlin R.L., 1977, MAGNETIC PROPERTIES
[6]   Er2Ti2O7:: Evidence of quantum order by disorder in a frustrated antiferromagnet -: art. no. 020401 [J].
Champion, JDM ;
Harris, MJ ;
Holdsworth, PCW ;
Wills, AS ;
Balakrishnan, G ;
Bramwell, ST ;
Cizmár, E ;
Fennell, T ;
Gardner, JS ;
Lago, J ;
McMorrow, DF ;
Orendác, M ;
Orendácová, A ;
Paul, DM ;
Smith, RI ;
Telling, MTF ;
Wildes, A .
PHYSICAL REVIEW B, 2003, 68 (02)
[7]   Soft modes in the easy plane pyrochlore antiferromagnet [J].
Champion, JDM ;
Holdsworth, PCW .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2004, 16 (11) :S665-S671
[8]   Absence of magnetic order in Yb3Ga5O12:: Relation between phase transition and entropy in geometrically frustrated materials -: art. no. 167201 [J].
de Réotier, PD ;
Yaouanc, A ;
Gubbens, PCM ;
Kaiser, CT ;
Baines, C ;
King, PJC .
PHYSICAL REVIEW LETTERS, 2003, 91 (16)
[9]   Muon spin relaxation investigation of the spin dynamics of geometrically frustrated antiferromagnets Y2Mo2O7 and Tb2Mo2O7 [J].
Dunsiger, SR ;
Kiefl, RF ;
Chow, KH ;
Gaulin, BD ;
Gingras, MJP ;
Greedan, JE ;
Keren, A ;
Kojima, K ;
Luke, GM ;
MacFarlane, WA ;
Raju, NP ;
Sonier, JE ;
Uemura, YJ ;
Wu, WD .
PHYSICAL REVIEW B, 1996, 54 (13) :9019-9022
[10]   SPIN-LATTICE RELAXATION IN CERIUM MAGNESIUM NITRATE AT LIQUID HELIUM TEMPERATURE - A NEW PROCESS [J].
FINN, CB ;
ORBACH, R ;
WOLF, WP .
PROCEEDINGS OF THE PHYSICAL SOCIETY OF LONDON, 1961, 77 (494) :261-&