Shear Melting of a Colloidal Glass

被引:65
作者
Eisenmann, Christoph [1 ]
Kim, Chanjoong [1 ]
Mattsson, Johan [1 ]
Weitz, David A. [1 ]
机构
[1] Harvard Univ, Dept Phys & HSEAS, Cambridge, MA 02138 USA
基金
美国国家科学基金会;
关键词
MODE-COUPLING THEORY; HARD-SPHERE; SUSPENSIONS; FLOW; TRANSITION; SOFT;
D O I
10.1103/PhysRevLett.104.035502
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We use confocal microscopy to explore shear melting of colloidal glasses, which occurs at strains of similar to 0.08, coinciding with a strongly non-Gaussian step size distribution. For larger strains, the particle mean square displacement increases linearly with strain and the step size distribution becomes Gaussian. The effective diffusion coefficient varies approximately linearly with shear rate, consistent with a modified Stokes-Einstein relationship in which thermal energy is replaced by shear energy and the length scale is set by the size of cooperatively moving regions consisting of similar to 3 particles.
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页数:4
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共 27 条
[1]   Three-dimensional imaging of colloidal glasses under steady shear [J].
Besseling, R. ;
Weeks, Eric R. ;
Schofield, A. B. ;
Poon, W. C. K. .
PHYSICAL REVIEW LETTERS, 2007, 99 (02)
[2]   Microstructure of strongly sheared suspensions and its impact on rheology and diffusion [J].
Brady, JF ;
Morris, JF .
JOURNAL OF FLUID MECHANICS, 1997, 348 :103-139
[3]   Universal nature of particle displacements close to glass and jamming transitions [J].
Chaudhuri, Pinaki ;
Berthier, Ludovic ;
Kob, Walter .
PHYSICAL REVIEW LETTERS, 2007, 99 (06)
[4]   Two-point microrheology of inhomogeneous soft materials [J].
Crocker, JC ;
Valentine, MT ;
Weeks, ER ;
Gisler, T ;
Kaplan, PD ;
Yodh, AG ;
Weitz, DA .
PHYSICAL REVIEW LETTERS, 2000, 85 (04) :888-891
[5]   Theory of nonlinear rheology and yielding of dense colloidal suspensions [J].
Fuchs, M ;
Cates, ME .
PHYSICAL REVIEW LETTERS, 2002, 89 (24)
[6]   A mode coupling theory for Brownian particles in homogeneous steady shear flow [J].
Fuchs, M. ;
Cates, M. E. .
JOURNAL OF RHEOLOGY, 2009, 53 (04) :957-1000
[7]   Direct observation of dynamical heterogeneities in colloidal hard-sphere suspensions [J].
Kegel, WK ;
van Blaaderen, A .
SCIENCE, 2000, 287 (5451) :290-293
[8]  
KRUGER M, 2009, THESIS U KONSTANZ
[9]   Nonlinear dynamics - Jamming is not just cool any more [J].
Liu, AJ ;
Nagel, SR .
NATURE, 1998, 396 (6706) :21-22
[10]   Nonlinear viscoelasticity of metastable complex fluids [J].
Miyazaki, K. ;
Wyss, H. M. ;
Weitz, D. A. ;
Reichman, D. R. .
EUROPHYSICS LETTERS, 2006, 75 (06) :915-921