All-inorganic lead halide perovskites: a promising choice for photovoltaics and detectors

被引：111
作者：
Deng, Jianping [1 ]
Li, Jinglei [2 ]
Yang, Zhi [2 ]
Wang, Minqiang [2 ]
机构：
[1] Shaanxi Univ Technol, Sch Mech Engn, Shaanxi Key Lab Ind Automat, Hanzhong 723001, Peoples R China
[2] Xi An Jiao Tong Univ, Sch Elect Sci & Engn, Shaanxi Engn Res Ctr Adv Energy Mat & Devices, ICDR,Key Lab Educ Minist,EMRL, Xian 710049, Shaanxi, Peoples R China
来源：
JOURNAL OF MATERIALS CHEMISTRY C | 2019年 / 7卷 / 40期
关键词：
LIGAND-MEDIATED SYNTHESIS; SOLAR-CELLS; QUANTUM DOTS; HIGH-EFFICIENCY; ALPHA-CSPBI3; PEROVSKITE; ENHANCED PERFORMANCE; ROOM-TEMPERATURE; SINGLE-CRYSTALS; CSPBBR3; PHOTODETECTORS;
D O I：
10.1039/c9tc04164h
中图分类号：
T [工业技术];
学科分类号：
08 ;
摘要：
Recent years have witnessed a significant performance breakthrough in all-inorganic perovskite solar cells, but their power conversion efficiencies are still far lower than the theoretical limit and they also suffer from severe moisture instability. Based on the discussions on crystal structures, chemical bonds, and optical and electrical properties of all-inorganic perovskites, we have summarized their comprehensive applications in solar cells and detectors. The effects of monovalent and divalent ion doping, morphology, crystallization control and interface engineering on device performance and stability have been carefully evaluated. A narrow-bandgap CsPbI3 polycrystalline bulk film solar cell has achieved the highest power conversion efficiency of 18.4%, while a stable CsPbBr3 nanocrystal film is a more successful choice in UV-visible and high-energy ray detections. Finally, we call on boosting the performance and stability of solar cells and shortening the response time for tandem photovoltaic and high-speed dynamic detection applications, respectively.
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收藏
页码：12415 / 12440
页数：26
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