MAX-DOAS measurements in southern China: retrieval of aerosol extinctions and validation using ground-based in-situ data

被引:68
作者
Li, X. [1 ,2 ]
Brauers, T. [1 ]
Shao, M. [2 ]
Garland, R. M. [3 ]
Wagner, T. [4 ]
Deutschmann, T. [5 ]
Wahner, A. [1 ]
机构
[1] Forschungszentrum Julich, Inst Chem & Dynam Geosphere ICG 2, D-52425 Julich, Germany
[2] Peking Univ, Coll Environm Sci & Engn, Beijing 100871, Peoples R China
[3] Max Planck Inst Chem, Biogeochem Dept, D-55128 Mainz, Germany
[4] Max Planck Inst Chem, Satellite Grp, D-55128 Mainz, Germany
[5] Univ Heidelberg, Inst Environm Phys, Heidelberg, Germany
关键词
OPTICAL-ABSORPTION SPECTROSCOPY; RADIATIVE-TRANSFER MODELS; CROSS-SECTIONS; TEMPERATURE-DEPENDENCE; SUN-PHOTOMETER; LIDAR; PROFILES; AIR; NM; FORMALDEHYDE;
D O I
10.5194/acp-10-2079-2010
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
We performed MAX-DOAS measurements during the PRiDe-PRD2006 campaign in the Pearl River Delta region 50 km north of Guangzhou, China, for 4 weeks in June 2006. We used an instrument sampling at 7 different elevation angles between 3 degrees and 90 degrees. During 9 cloud-free days, differential slant column densities (DSCDs) of O-4 (O-2 dimer) absorptions between 351 nm and 389 nm were evaluated for 6 elevation angles. Here, we show that radiative transfer modeling of the DSCDS can be used to retrieve the aerosol extinction and the height of the boundary layer. A comparison of the aerosol extinction with simultaneously recorded, ground based nephelometer data shows excellent agreement.
引用
收藏
页码:2079 / 2089
页数:11
相关论文
共 34 条
[21]   Influences of relative humidity and particle chemical composition on aerosol scattering properties during the 2006 PRD campaign [J].
Liu, Xingang ;
Cheng, Yafang ;
Zhang, Yuanhang ;
Jung, Jinsang ;
Sugimoto, Nobuo ;
Chang, Shih-Yu ;
Kim, Young J. ;
Fan, Shaojia ;
Zeng, Limin .
ATMOSPHERIC ENVIRONMENT, 2008, 42 (07) :1525-1536
[22]   Temperature dependence of the absorption cross sections of formaldehyde between 223 and 323 K in the wavelength range 225-375 nm [J].
Meller, R ;
Moortgat, GK .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2000, 105 (D6) :7089-7101
[23]   Intercomparison of multiaxis and long-path differential optical absorption spectroscopy measurements in the marine boundary layer [J].
Pikelnaya, Olga ;
Hurlock, Stephen C. ;
Trick, Sebastian ;
Stutz, Jochen .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2007, 112 (D10)
[24]   Corrections for zenith scattered light DOAS [J].
Platt, U ;
Marquard, L ;
Wagner, T ;
Perner, D .
GEOPHYSICAL RESEARCH LETTERS, 1997, 24 (14) :1759-1762
[25]  
Platt U, 2008, PHYS EARTH SPACE ENV, P1, DOI 10.1007/978-3-540-75776-4_1
[26]   Tropospheric aerosol extinction coefficient profiles derived from scanning lidar measurements over Tsukuba, Japan, from 1990 to 1993 [J].
Sasano, Y .
APPLIED OPTICS, 1996, 35 (24) :4941-4952
[27]   MAX-DOAS detection of glyoxal during ICARTT 2004 [J].
Sinreich, R. ;
Filsinger, F. ;
Friess, U. ;
Platt, U. ;
Sebastian, O. ;
Wagner, T. ;
Volkamer, R. ;
Kern, C. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 :1293-1303
[28]   The temperature and pressure dependence of the absorption cross-sections of NO2 in the 250-800 nm region measured by Fourier-transform spectroscopy [J].
Voigt, S ;
Orphal, J ;
Burrows, JP .
JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 2002, 149 (1-3) :1-7
[29]   The temperature dependence (203-293 K) of the absorption cross sections of O3 in the 230-850 nm region measured by Fourier-transform spectroscopy [J].
Voigt, S ;
Orphal, J ;
Bogumil, K ;
Burrows, JP .
JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY A-CHEMISTRY, 2001, 143 (01) :1-9
[30]   Comparison of box-air-mass-factors and radiances for Multiple-Axis Differential Optical Absorption Spectroscopy (MAX-DOAS) geometries calculated from different UV/visible radiative transfer models [J].
Wagner, T. ;
Burrows, J. P. ;
Deutschmann, T. ;
Dix, B. ;
von Friedeburg, C. ;
Friess, U. ;
Hendrick, F. ;
Heue, K. -P. ;
Irie, H. ;
Iwabuchi, H. ;
Kanaya, Y. ;
Keller, J. ;
McLinden, C. A. ;
Oetjen, H. ;
Palazzi, E. ;
Petritoli, A. ;
Platt, U. ;
Postylyakov, O. ;
Pukite, J. ;
Richter, A. ;
van Roozendael, M. ;
Rozanov, A. ;
Rozanov, V. ;
Sinreich, R. ;
Sanghavi, S. ;
Wittrock, F. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2007, 7 (07) :1809-1833