Preparation of a novel sonocatalyst, Au/NiGa2O4-Au-Bi2O3 nanocomposite, and application in sonocatalytic degradation of organic pollutants

被引:48
作者
Wang, Guowei [1 ]
Huang, Yingying [1 ]
Li, Guanshu [2 ]
Zhang, Hongbo [1 ]
Wang, Yidi [2 ]
Li, Bowen [2 ]
Wang, Jun [1 ,2 ]
Song, Youtao [2 ]
机构
[1] Liaoning Univ, Coll Chem, Shenyang 110036, Peoples R China
[2] Liaoning Univ, Coll Environm, Shenyang 110036, Peoples R China
基金
美国国家科学基金会;
关键词
Preparation; Au/NiGa2O4-Au-Bi2O3; composite; Organic pollutants; Sonocatalytic degradation; ACRYLAMIDE-GEL METHOD; PHOTOCATALYTIC DEGRADATION; ULTRASONIC IRRADIATION; HYDROXYL RADICALS; ACTIVATED-SLUDGE; WASTE-WATER; SONOLUMINESCENCE; COMPOSITE; NANOPARTICLES; PERFORMANCE;
D O I
10.1016/j.ultsonch.2017.03.031
中图分类号
O42 [声学];
学科分类号
070206 ; 082403 ;
摘要
A novel nanocomposite, Au/NiGa2O4-Au-Bi2O3, as an effective sonocatalyst was prepared through hydrothermal process and high-temperature calcination methods, and then characterized by X-ray diffractometer (XRD), scanning electron microscopy (SEM) and energy dispersive X-ray spectroscopy (EDX). The sonocatalytic activity of Au/NiGa2O4-Au-Bi2O3 nanocomposite was detected through the degradation of some organic pollutants under ultrasonic irradiation. Furthermore, the influences of mass ratio of NiGa2O4 and Bi2O3, ultrasonic irradiation time and used times on the sonocatalytic degradation efficiency were investigated by using Total Organic Carbon (TOC) and UV-vis spectroscopy. The experimental results showed that, because of the existence of Au nanoparticles (AuNPs) served as both conductive passageway and co-catalyst, the nanocomposite sonocatalyst (Au/NiGa2O4-Au-Bi2O3) displayed an excellent sonocatalytic activity in degradation of some organic pollutants under ultrasonic irradiation. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:335 / 346
页数:12
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