The fate of polycyclic aromatic hydrocarbons (PAHs) and organochlorine pesticides (OCPs) in water from Poyang Lake, the largest freshwater lake in China

被引:110
作者
Zhi, Hui [1 ]
Zhao, Zhonghua [2 ]
Zhang, Lu [2 ]
机构
[1] Cornell Univ, Sch Engn, Dept Civil & Environm Engn, Ithaca, NY 14853 USA
[2] Chinese Acad Sci, Nanjing Inst Geog & Limnol, State Key Lab Lake Sci & Environm Res, Nanjing 210008, Jiangsu, Peoples R China
基金
美国国家科学基金会;
关键词
Organochlorine pesticides; Polycyclic aromatic hydrocarbons; Poyang Lake; Spatial distribution; Source identification; PERSISTENT ORGANIC POLLUTANTS; MINJIANG-RIVER-ESTUARY; SOUTH CHINA; QIANTANG RIVER; PEARL RIVER; SARNO RIVER; SEDIMENTS; CONTAMINATION; DEGRADATION; POLLUTION;
D O I
10.1016/j.chemosphere.2014.09.054
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The fate of polycyclic hydrocarbons (PAHs) and organochlorine pesticides (OCPs) in the water columns from Poyang Lake was studied. The total concentrations of OCPs and PAHs were 19.10-111.78 ng L-1 and 5.56-266.1 ng L-1, respectively. Among OCPs, endosulfans, chlordanes, and HCHs accounted for 21.96%, 24,6% and 24.65%, and were the predominant pollutants. Results suggested that the main sources of DDTs were residue from technical DDTs and dicofol, as well as antifouling paints for ships, while for HCHs, the main sources included long-distance transmission, agriculture activities and the combination of industrial products with separate lindane in use. As for PAHs, the predominance of lower molecular weight congeners demonstrated that petroleum and the combustion products of fuel oil, as well as other pyrogenic sources, contributed to the main input of PAHs in the Poyang region. The vehicle emissions were mostly from diesel engines. Moreover, HCH, DDT and BaP concentrations in water of Poyang Lake were all below the threshold values. Crown Copyright (C) 2014 Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:1134 / 1140
页数:7
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