Porous metal-organic frameworks for fuel storage

被引:217
作者
He, Yabing [1 ]
Chen, Fengli [1 ]
Li, Bin [2 ]
Qian, Guodong [2 ]
Zhou, Wei [3 ]
Chen, Banglin [1 ,4 ]
机构
[1] Zhejiang Normal Univ, Coll Chem & Life Sci, Jinhua 321004, Peoples R China
[2] Zhejiang Univ, Dept Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China
[3] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA
[4] Univ Texas San Antonio, Dept Chem, One UTSA Circle, San Antonio, TX 78249 USA
关键词
Metal-organic frameworks; Methane storage; Acetylene storage; Gas adsorption; HIGH METHANE STORAGE; HIGH H-2 ADSORPTION; HIGH-SURFACE-AREA; GAS-ADSORPTION; HIGH ACETYLENE; HIGH-CAPACITY; C2H2; STORAGE; COORDINATION COPOLYMER; ISOPHTHALATE LINKERS; SELECTIVE ADSORPTION;
D O I
10.1016/j.ccr.2017.10.002
中图分类号
O61 [无机化学];
学科分类号
070301 ; 081704 ;
摘要
Methane and acetylene represent cleaner fuels, which are considered as ideal alternatives to fossil fuels. Due to low volumetric energy density at ambient conditions, it is highly desirable to develop porous materials such as metal-organic frameworks that exhibit good adsorption properties with respect to them. In this review, we firstly introduced the development history on the design and synthesis of porous metal-organic frameworks for acetylene and methane storage in which some representative examples were analyzed; and then we focused on discussing their adsorption mechanisms including the gas binding sites and gas-framework interactions. At last, some structure-property relationships and synthetic strategies for improving gas adsorption properties with respect to them were summarized. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:167 / 198
页数:32
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