Integrated process for the removal of indoor VOCs from food industry manufacturing: Elimination of Butane-2,3-dione and Heptan-2-one by cold plasma-photocatalysis combination

被引:34
作者
Abou Saoud, Wala [1 ]
Assadi, Aymen Amine [1 ]
Kane, Abdoulaye [2 ]
Jung, Aude-Valerie [2 ]
Le Cann, Pierre [3 ]
Gerard, Anne [3 ]
Bazantay, Frederic [4 ]
Bouzaza, Abdelkrim [1 ]
Wolbert, Dominque [1 ]
机构
[1] Univ Rennes, Ecole Natl Super Chimie Rennes, CNRS, ISCR,UMR 6226, F-35000 Rennes, France
[2] UniLaSalle Ecole Metiers Environm UniLaSalle EME, Campus Ker Lann,Ave Robert Schuman, Bruz, France
[3] Univ Rennes, UMR S 1085, INSERM, EHESP,Irset, F-35000 Rennes, France
[4] Pole Cristo, 49 Ave Rene Cassin, F-22100 Dinan, France
关键词
Indoor air of food industry; Butane-2,3-dione/Heptan-2-one mixture; (Photocatalysis-DBD plasma) association; Synergetic effect; DIELECTRIC BARRIER DISCHARGE; CONTINUOUS REACTOR; NONTHERMAL PLASMA; GAS-PHASE; OXIDATION; ABATEMENT;
D O I
10.1016/j.jphotochem.2019.112071
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Coupling Non-thermal plasma (dielectric barrier discharge) with photocatalysis (TiO2-/UV) can be a promising technique to improve indoor air quality. In this study, Butane-2,3-dione and Heptan-2-one, usually found in food industry, were used as target compounds. Firstly, each pollutant was studied alone by photocatalytic treatment under experimental parameter effects like gases flow rate, VOCs inlet concentration, and humidity levels. Otherwise, in order to understand pollutants reaction mechanisms, a complex composition mixture was then studied and discussed. Experiments with dry and wet air showed good Heptan-2-one removal but negatively affected Butane-2,3-dione elimination rate. The Butane-2,3-dione/Heptan-2-one oxidation study was carried out by cold plasma-photocatalysis combination in the same pilot reactor. Excellent treatment yields were observed in terms of pollutant removal efficiency, mineralization and Ozone decomposition. Additionally, intermediate by-product exhausts from three technologies e.g. TiO2/UV-light system, DBD-plasma and their combination are identified.
引用
收藏
页数:9
相关论文
共 35 条
[1]   Photocatalytic indoor/outdoor air treatment and bacterial inactivation on CuxO/TiO2 prepared by HiPIMS on polyester cloth under low intensity visible light [J].
Abidi, M. ;
Assadi, A. A. ;
Bouzaza, A. ;
Hajjaji, A. ;
Bessais, B. ;
Rtimi, S. .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2019, 259
[2]   Synergism between non-thermal plasma and photocatalysis: Implicationsin the post discharge of ozone at a pilot scale in a catalytic fixed-bed reactor [J].
Abou Saoud, Wala ;
Assadi, Aymen Amine ;
Guiza, Monia ;
Loganathan, Sivachandiran ;
Bouzaza, Abdelkrim ;
Aboussaoud, Wael ;
Ouederni, Abdelmottaleb ;
Rtimi, Sami ;
Wolbert, Dominique .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2019, 241 :227-235
[3]   Abatement of ammonia and butyraldehyde under non-thermal plasma and photocatalysis: Oxidation processes for the removal of mixture pollutants at pilot scale [J].
Abou Saoud, Wala ;
Assadi, Aymen Amine ;
Guiza, Monia ;
Bouzaza, Abdelkrim ;
Aboussaoud, Wael ;
Soutrel, Isabelle ;
Ouederni, Abdelmottaleb ;
Wolbert, Dominique ;
Rtimi, Sami .
CHEMICAL ENGINEERING JOURNAL, 2018, 344 :165-172
[4]   Study of synergetic effect, catalytic poisoning and regeneration using dielectric barrier discharge and photocatalysis in a continuous reactor: Abatement of pollutants in air mixture system [J].
Abou Saoud, Wala ;
Assadi, Aymen Amine ;
Guiza, Monia ;
Bouzaza, Abdelkrim ;
Aboussaoud, Wael ;
Ouederni, Abdelmottaleb ;
Soutrel, Isabelle ;
Wolbert, Dominique ;
Rtimi, Sami .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2017, 213 :53-61
[5]   A parametric study of the UV-A photocatalytic oxidation of H2S over TiO2 [J].
Alonso-Tellez, Angela ;
Robert, Didier ;
Keller, Nicolas ;
Keller, Valerie .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2012, 115 :209-218
[6]   Pilot scale degradation of mono and multi volatile organic compounds by surface discharge plasma/TiO2 reactor: Investigation of competition and synergism [J].
Assadi, Aymen Amine ;
Loganathan, Sivachandiran ;
Phuong Nguyen Tri ;
Ghaida, Sara Gharib-Abou ;
Bouzaza, Abdelkrim ;
Anh Nguyen Tuan ;
Wolbert, Dominique .
JOURNAL OF HAZARDOUS MATERIALS, 2018, 357 :305-313
[7]   A study of pollution removal in exhaust gases from animal quartering centers by combining photocatalysis with surface discharge plasma: From pilot to industrial scale [J].
Assadi, Aymen Amine ;
Bouzaza, Abdelkrim ;
Soutrel, Isabelle ;
Petit, Philippe ;
Medimagh, Karim ;
Wolbert, Dominique .
CHEMICAL ENGINEERING AND PROCESSING-PROCESS INTENSIFICATION, 2017, 111 :1-6
[8]   Comparative study between laboratory and large pilot scales for VOC's removal from gas streams in continuous flow surface discharge plasma [J].
Assadi, Aymen Amine ;
Bouzaza, Abdelkrim ;
Wolbert, Dominique .
CHEMICAL ENGINEERING RESEARCH & DESIGN, 2016, 106 :308-314
[9]   Impact of design parameters on the performance of non-thermal plasma air purification system [J].
Bahri, Mitra ;
Haghighat, Fariborz ;
Rohani, Sohrab ;
Kazemian, Hossein .
CHEMICAL ENGINEERING JOURNAL, 2016, 302 :204-212
[10]   Occurrence of 13 volatile organic compounds in foods from the Canadian total diet study [J].
Cao, Xu-Liang ;
Sparling, Melissa ;
Dabeka, Robert .
FOOD ADDITIVES AND CONTAMINANTS PART A-CHEMISTRY ANALYSIS CONTROL EXPOSURE & RISK ASSESSMENT, 2016, 33 (02) :373-382