Graphene-based materials: Synthesis and gas sorption, storage and separation

被引:598
作者
Gadipelli, Srinivas [1 ]
Guo, Zheng Xiao [1 ]
机构
[1] UCL, Dept Chem, London WC1H 0AJ, England
基金
英国工程与自然科学研究理事会;
关键词
Graphene; Graphene oxide; Synthesis; Hydrogen storage; Methane storage; Carbon capture; Gas storage; Gas separation; NITROGEN-DOPED GRAPHENE; METAL-ORGANIC FRAMEWORK; CARBON-DIOXIDE CAPTURE; HIGH-SURFACE-AREA; ZEOLITIC-IMIDAZOLATE-FRAMEWORK; ELECTROCHEMICAL HYDROGEN STORAGE; HIERARCHICALLY POROUS CARBON; BORON-SUBSTITUTED GRAPHENE; CALCIUM-DECORATED GRAPHENE; SINGLE-LAYER GRAPHENE;
D O I
10.1016/j.pmatsci.2014.10.004
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Graphene-based materials have generated tremendous interest in a wide range of research activities. A wide variety of graphene related materials have been synthesised for potential applications in electronics, energy storage, catalysis, and gas sorption, storage, separation and sensing. Recently, gas sorption, storage and separation in porous nanocarbons and metal-organic frameworks have received increasing attention. In particular, the tuneable porosity, surface area and functionality of the lightweight and stable graphene-based materials open up great scope for those applications. Such structural features can be achieved by the design and control of the synthesis routes. Here, we highlight recent progresses and challenges in the syntheses of graphene-based materials with hierarchical pore structures, tuneable high surface area, chemical doping and surface functionalization for gas (H-2, CH4, CO2, N-2, NH3, NO2, H2S, SO2, etc.) sorption, storage and separation. (C) 2014 The Authors. Published by Elsevier Ltd.
引用
收藏
页码:1 / 60
页数:60
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