Cross Section Measurement Method for (n, α) Reaction of Gas Sample Based on Combination of Experiment and Simulation

被引:0
作者
Hu Y. [1 ]
Cui Z. [1 ]
Liu J. [1 ]
Bai H. [1 ]
Xia C. [1 ]
Jiang H. [1 ]
Chen J. [1 ]
Zhang G. [1 ]
机构
[1] State Key Laboratory of Nuclear Physics and Technology, Institute of Heavy Ion Physics, School of Physics, Peking University, Beijing
来源
Yuanzineng Kexue Jishu/Atomic Energy Science and Technology | 2022年 / 56卷 / 05期
关键词
(n; reaction; Gas sample; Gridded ionization chamber; Resonance cross section;
D O I
10.7538/yzk.2022.youxian.0110
中图分类号
学科分类号
摘要
A method for measuring (n, α) reaction cross sections of the gas sample induced by fast neutrons using a gridded ionization chamber (GIC) was established. There are several advantages using the GIC to measure gas samples. With this method, the (n, α) reaction cross sections of inert gases which are hard to exist as a solid can be measured. And the (n, α) reaction cross section for α particle emitting in all directions can be directly measured by using the gas sample. Furthermore, compared with using solid samples, using gas samples have far more nuclei in the measurement samples. Therefore, it is feasible to use neutron source with a better energy resolution to measure the resonance cross sections with gas sample. However, there are many problems to be solved when measuring (n, α) reaction cross section of gas sample by using the GIC. On the one hand, the nuclear reaction event will be affected by the wall effect, when the nuclear reaction is generated near the electrodes of the GIC or at the edge of the electric field. The wall effect will cause the measured event to locate outside the event area which cannot be counted. Not only is the number of nuclei of the gas samples involved in the (n, α) reaction difficult to determine, but the number of events, which are affected by the background or located below the threshold, is also difficult to count. On the other hand, the neutron fluence involved in the measurement of (n, α) reaction cross section of gas sample is difficult to measure. Aiming at solving the problems of the determination of the sample nuclei number, the measurement of neutron fluence, and the selection of events, which are all difficult for the gas sample, this method included three steps: First, simulation calculation was performed to select a suitable effective volume of the gas samples, so that the event is free of background and easy to be counted. Second, the neutron collimator and the timing information of cathode and anode signals were used to select and count the events generated in the effective volume of the gas sample. Third, combining the fission fragment measurement of the 238U(n, f) reaction and the simulation based on SuperMC, the neutron fluence through the effective volume was obtained. Measurements of relative cross sections of the 14N(n, α0) reaction using gas sample were performed at En=4.71, 4.87, 5.00, 5.12, 5.29, and 5.45 MeV. The results are in good agreement with those of ENDF/B-Ⅷ.0 which verified the present measurement method. © 2022, Editorial Board of Atomic Energy Science and Technology. All right reserved.
引用
收藏
页码:825 / 834
页数:9
相关论文
共 28 条
[1]  
RAFLIS H, MUHAMMAD I, SU'UD Z, Et al., Reflector materials selection for core design of modular gas-cooled fast reactor using OpenMC code, International Journal of Energy Research, 45, 8, pp. 12071-12085, (2021)
[2]  
YANG Maochun, A case of noble gas leak age searching and analysis in dayabay NPP, Radialization Protection, 19, 5, pp. 386-391, (1999)
[3]  
SANAMI T, BABA M, SAITO K, Et al., (n, α) cross-section measurement using a gaseous sample and a gridded ionization chamber, Nuclear Instruments and Methods in Physics Research A, 440, 2, pp. 403-408, (2000)
[4]  
SANAMI T, BABA M, SAITO K, Et al., (n, α) cross section measurement of light nuclei using gridded ionization chamber and gaseous sample, pp. 192-197, (1998)
[5]  
BABA M, TAKADA M, IWASAKI T, Et al., Development of monoenergetic neutron calibration fields between 8 keV and 15 MeV, Nuclear Instruments and Methods in Physics Research A, 376, 1, pp. 115-123, (1996)
[6]  
KHRYACHKOV V A, KUZ'MINOV B D, DUNAEV M V, Et al., Measurement of the cross sections of the reactions <sup>14</sup>N(n, α)<sup>11</sup>B and <sup>14</sup>N(n, t)<sup>12</sup>C at neutron energies 5.45-7.2 MeV, Atomic Energy, 101, 4, pp. 760-765, (2006)
[7]  
KHRYACHKOV V A, BONDARENKO I P, KUZMINOV B D, Et al., (n, α) reactions cross section research at IPPE, EPJ Web of Conferences, 21, (2012)
[8]  
KHRYACHKOV V A, BONDARENKO I P, KUZMINOV B D, Et al., Measurement of the cross section for the reaction <sup>20</sup>Ne(n, α)<sup>17</sup>O in the neutron-energy between 4 and 7 MeV, Physics of Atomic Nuclei, 75, 4, pp. 404-410, (2012)
[9]  
BONDARENKO I P, KHRYACHKOV V A, IVANOVA T A, Et al., Investigation of the <sup>19</sup>F(n, α)<sup>16</sup>N reaction excitation function in neutron energy range of 4-7.35 MeV, Bulletin of the Russian Academy of Sciences: Physics, 77, 4, pp. 459-461, (2013)
[10]  
JIANG H, CUI Z, HU Y, Et al., Cross-section measurements for <sup>58, 60, 61</sup>Ni(n, α)<sup>55, 57, 58</sup>Fe reactions in the 4.50-5.50 MeV neutron energy region, Chinese Physics C, 44, 11, (2020)