Construction of 2D/2D Heterogeneous of ZIF-8/SnS2 Composite as a Transfer of Band-Band System for Efficient Visible Photocatalytic Activity

被引:13
作者
Chou, Xiaoyu [1 ]
Ye, Jin [2 ]
Cui, Mimi [2 ]
Li, Yudong [3 ]
He, Yanzhen [2 ]
Liu, Xiaofei [1 ]
Wang, Hongchao [4 ]
机构
[1] Hulunbuir Univ, Coll Chem & Chem Engn, Hulunbuir 021008, Inner Mongolia, Peoples R China
[2] Hebei Univ Technol, Inst Polymer Sci & Engn, Tianjin 300130, Peoples R China
[3] Northeast Forestry Univ, Key Lab Biobased Mat Sci & Technol, Minist Educ, Harbin 150040, Heilongjiang, Peoples R China
[4] Xiamen Univ, Coll Mat, Xiamen 361000, Fujian, Peoples R China
关键词
2D-ZIF-8; SnS2; Heterojunction; Photocatalysis; Visible-light-driven; MICROWAVE-ASSISTED SYNTHESIS; METAL-ORGANIC FRAMEWORK; Z-SCHEME PHOTOCATALYST; LIGHT IRRADIATION; HIGHLY EFFICIENT; SNS2; NANOSHEETS; FACILE FABRICATION; CHARGE SEPARATION; HYDROGEN STORAGE; RATIONAL DESIGN;
D O I
10.1002/slct.201902494
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Constructing two-dimensional (2D) heterostructured nanocomposites is an effective method to boost photo-generated carrier separation efficiently using layer material. In this work, a tightly coupled 2D/2D ZIF-8/SnS2 nanosheet heterogeneous composite was successfully prepared. Due to the good heterogeneous interface between 2D SnS2 and 2D ZIF-8 nanosheet, 2D/2D ZIF-8/SnS2 nanocomposites formed a large contact interface, leading to high efficient interfacial charge transfer efficiency and shortening the distance of charge transmission. As a result, the optimized SnS2/2D-ZIF-8 composites possess excellent photocatalytic properties and the rate of degradation toward MB under visible light for 100 minutes is 2.32 and 26.75 times than that of pure SnS2 and 2D-ZIF-8, respectively. This work offers an efficient way to design 2D/2D heterojunction composites as visible-light-driven catalyst for the photocatalytic application.
引用
收藏
页码:11227 / 11234
页数:8
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