Nanocrystal Quantum Dots: From Discovery to Modern Development

被引：411

作者：

Efros, Alexander L. ^{[2
]}

Brus, Louis E. ^{[1
]}

机构：

[1] Columbia Univ, Dept Chem, New York, NY 10027 USA

[2] Naval Res Lab, Ctr Computat Mat Sci, Washington, DC 20375 USA

来源：

ACS NANO | 2021年 / 15卷 / 04期

基金：

美国国家科学基金会;

关键词：

nanocrystals; quantum dots; quantum dot synthesis; colloid; exciton; quantum size effect; core-shell structures; liquid crystal display; light-emitting diodes; solar cells; EXCITED ELECTRONIC STATES; SEMICONDUCTOR NANOCRYSTALS; MULTIEXCITON GENERATION; OPTICAL-PROPERTIES; CATION-EXCHANGE; CDS PARTICLES; STRUCTURAL-CHARACTERIZATION; CORE/SHELL NANOCRYSTALS; COLLOIDAL NANOCRYSTALS; SIZE QUANTIZATION;

D O I：

10.1021/acsnano.1c01399

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

This review traces nanocrystal quantum dot (QD) research from the early discoveries to the present day and into the future. We describe the extensive body of theoretical and experimental knowledge that comprises the modern science of QDs. Indeed, the spatial confinement of electrons, holes, and excitons in nanocrystals, coupled with the ability of modern chemical synthesis to make complex designed structures, is today enabling multiple applications of QD size-tunable electronic and optical properties.

引用

页码：6192 / 6210

页数：19

共 183 条

[1] Impact of Shell Growth on Recombination Dynamics and Exciton-Phonon Interaction in CdSe-CdS Core-Shell Nanoplatelets [J].

Achtstein, Alexander W. ;

Marquardt, Oliver ;

Scott, Riccardo ;

Ibrahim, Mohamed ;

Riedl, Thomas ;

Prudnikau, Anatol, V ;

Antanovich, Artsiom ;

Owschimikow, Nina ;

Lindner, Joerg K. N. ;

Artemyev, Mikhail ;

Woggon, Ulrike .

ACS NANO, 2018, 12 (09) :9476-9483

[2] ELECTRON-VIBRATION COUPLING IN SEMICONDUCTOR CLUSTERS STUDIED BY RESONANCE RAMAN-SPECTROSCOPY [J].

ALIVISATOS, AP ;

HARRIS, TD ;

CARROLL, PJ ;

STEIGERWALD, ML ;

BRUS, LE .

JOURNAL OF CHEMICAL PHYSICS, 1989, 90 (07) :3463-3468

[3] ELECTRONIC STATES OF SEMICONDUCTOR CLUSTERS - HOMOGENEOUS AND INHOMOGENEOUS BROADENING OF THE OPTICAL-SPECTRUM [J].

ALIVISATOS, AP ;

HARRIS, AL ;

LEVINOS, NJ ;

STEIGERWALD, ML ;

BRUS, LE .

JOURNAL OF CHEMICAL PHYSICS, 1988, 89 (07) :4001-4011

[4] Expeditious Stochastic Calculation of Multiexciton Generation Rates in Semiconductor Nanocrystals [J].

Baer, Roi ;

Rabani, Eran .

NANO LETTERS, 2012, 12 (04) :2123-2128

[5]

Banyai L., 1993, Semiconductor Quantum Dots, V2

[6] Electronic states and optical properties of PbSe nanorods and nanowires [J].

Bartnik, A. C. ;

Efros, Al. L. ;

Koh, W. -K. ;

Murray, C. B. ;

Wise, F. W. .

PHYSICAL REVIEW B, 2010, 82 (19)

[7] Formation of high quality InP and InAs nanocrystals in a noncoordinating solvent [J].

Battaglia, D ;

Peng, XG .

NANO LETTERS, 2002, 2 (09) :1027-1030

[8] THE QUANTUM-MECHANICS OF LARGER SEMICONDUCTOR CLUSTERS (QUANTUM DOTS) [J].

BAWENDI, MG ;

STEIGERWALD, ML ;

BRUS, LE .

ANNUAL REVIEW OF PHYSICAL CHEMISTRY, 1990, 41 :477-496

[9] X-RAY STRUCTURAL CHARACTERIZATION OF LARGER CDSE SEMICONDUCTOR CLUSTERS [J].

BAWENDI, MG ;

KORTAN, AR ;

STEIGERWALD, ML ;

BRUS, LE .

JOURNAL OF CHEMICAL PHYSICS, 1989, 91 (11) :7282-7290

[10] ELECTRONIC-STRUCTURE AND PHOTOEXCITED-CARRIER DYNAMICS IN NANOMETER-SIZE CDSE CLUSTERS [J].

BAWENDI, MG ;

WILSON, WL ;

ROTHBERG, L ;

CARROLL, PJ ;

JEDJU, TM ;

STEIGERWALD, ML ;

BRUS, LE .

PHYSICAL REVIEW LETTERS, 1990, 65 (13) :1623-1626

← 1 2 3 4 5 6 7 8 9 10 →