ITO-free highly bendable and efficient organic solar cells with Ag nanomesh/ZnO hybrid electrodes

被引:58
作者
Song, Myungkwan [1 ]
Kim, Han-Jung [2 ]
Kim, Chang Su [1 ]
Jeong, Jun-Ho [2 ]
Cho, Changsoon [3 ]
Lee, Jung-Yong [3 ]
Jin, Sung-Ho [4 ]
Choi, Dae-Geun [2 ]
Kim, Dong-Ho [1 ]
机构
[1] Korea Inst Mat Sci, Adv Funct Thin Films Dept, Chang Won 641831, South Korea
[2] KIMM, Nanomech Syst Res Div, Taejon 305343, South Korea
[3] Korea Adv Inst Sci & Technol, Grad Sch Energy Environm Water & Sustainabil EEWS, Taejon 305701, South Korea
[4] Pusan Natl Univ, Inst Plast Informat & Energy Mat, Grad Dept Chem Mat, Dept Chem Educ, Pusan 609735, South Korea
基金
新加坡国家研究基金会;
关键词
TO-ROLL PRODUCTION; TRANSPARENT; FILMS; CONDUCTIVITY;
D O I
10.1039/c4ta05294c
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We demonstrate a facile approach to fabricate Ag nanomesh transparent conducting electrodes (TCEs) on a flexible substrate using nanoimprint lithography (NIL) and transfer printing without a conducting polymer. The Ag nanomesh TCEs exhibited a high transmittance of similar to 88% and a low sheet resistance of similar to 15 Omega sq(-1) as well as superior mechanical flexibility. Furthermore, flexible inverted organic solar cells (IOSCs) with Ag nanomesh TCEs exhibited a power conversion efficiency (PCE) of similar to 7.15% under 100 mW cm (2) AM 1.5G illumination as well as superior long-term stability under ambient conditions. This type of highly flexible and transparent Ag nanomesh electrode is a promising candidate for use with TCEs in various optoelectronic devices.
引用
收藏
页码:65 / 70
页数:6
相关论文
共 45 条
[11]   Effective Work Function Modulation of Graphene/Carbon Nanotube Composite Films As Transparent Cathodes for Organic Optoelectronics [J].
Huang, Jen-Hsien ;
Fang, Jheng-Hao ;
Liu, Chung-Chun ;
Chu, Chih-Wei .
ACS NANO, 2011, 5 (08) :6262-6271
[12]   Nanoimprinted semitransparent metal electrodes and their application in organic light-emitting diodes [J].
Kang, Myung-Gyu ;
Guo, L. Jay .
ADVANCED MATERIALS, 2007, 19 (10) :1391-+
[13]   Organic Solar Cells Using Nanoimprinted Transparent Metal Electrodes [J].
Kang, Myung-Gyu ;
Kim, Myung-Su ;
Kim, Jinsang ;
Guo, L. Jay .
ADVANCED MATERIALS, 2008, 20 (23) :4408-4413
[14]   High-Concentration Solvent Exfoliation of Graphene [J].
Khan, Umar ;
O'Neill, Arlene ;
Lotya, Mustafa ;
De, Sukanta ;
Coleman, Jonathan N. .
SMALL, 2010, 6 (07) :864-871
[15]   Large-scale pattern growth of graphene films for stretchable transparent electrodes [J].
Kim, Keun Soo ;
Zhao, Yue ;
Jang, Houk ;
Lee, Sang Yoon ;
Kim, Jong Min ;
Kim, Kwang S. ;
Ahn, Jong-Hyun ;
Kim, Philip ;
Choi, Jae-Young ;
Hong, Byung Hee .
NATURE, 2009, 457 (7230) :706-710
[16]   Achieving High Efficiency and Improved Stability in ITO-Free Transparent Organic Light-Emitting Diodes with Conductive Polymer Electrodes [J].
Kim, Yong Hyun ;
Lee, Jonghee ;
Hofmann, Simone ;
Gather, Malte C. ;
Mueller-Meskamp, Lars ;
Leo, Karl .
ADVANCED FUNCTIONAL MATERIALS, 2013, 23 (30) :3763-3769
[17]   Analysis of the failure mechanism for a stable organic photovoltaic during 10000 h of testing [J].
Krebs, Frederik C. ;
Norrman, Kion .
PROGRESS IN PHOTOVOLTAICS, 2007, 15 (08) :697-712
[18]   25th Anniversary Article: Rise to Power - OPV-Based Solar Parks [J].
Krebs, Frederik C. ;
Espinosa, Nieves ;
Hosel, Markus ;
Sondergaard, Roar R. ;
Jorgensen, Mikkel .
ADVANCED MATERIALS, 2014, 26 (01) :29-39
[19]   Product integration of compact roll-to-roll processed polymer solar cell modules: methods and manufacture using flexographic printing, slot-die coating and rotary screen printing [J].
Krebs, Frederik C. ;
Fyenbo, Jan ;
Jorgensen, Mikkel .
JOURNAL OF MATERIALS CHEMISTRY, 2010, 20 (41) :8994-9001
[20]   Upscaling of polymer solar cell fabrication using full roll-to-roll processing [J].
Krebs, Frederik C. ;
Tromholt, Thomas ;
Jorgensen, Mikkel .
NANOSCALE, 2010, 2 (06) :873-886