ITO-free highly bendable and efficient organic solar cells with Ag nanomesh/ZnO hybrid electrodes

被引：58

作者：

Song, Myungkwan ^{[1
]}

Kim, Han-Jung ^{[2
]}

Kim, Chang Su ^{[1
]}

Jeong, Jun-Ho ^{[2
]}

Cho, Changsoon ^{[3
]}

Lee, Jung-Yong ^{[3
]}

Jin, Sung-Ho ^{[4
]}

Choi, Dae-Geun ^{[2
]}

Kim, Dong-Ho ^{[1
]}

机构：

[1] Korea Inst Mat Sci, Adv Funct Thin Films Dept, Chang Won 641831, South Korea

[2] KIMM, Nanomech Syst Res Div, Taejon 305343, South Korea

[3] Korea Adv Inst Sci & Technol, Grad Sch Energy Environm Water & Sustainabil EEWS, Taejon 305701, South Korea

[4] Pusan Natl Univ, Inst Plast Informat & Energy Mat, Grad Dept Chem Mat, Dept Chem Educ, Pusan 609735, South Korea

来源：

JOURNAL OF MATERIALS CHEMISTRY A | 2015年 / 3卷 / 01期

基金：

新加坡国家研究基金会;

关键词：

TO-ROLL PRODUCTION; TRANSPARENT; FILMS; CONDUCTIVITY;

D O I：

10.1039/c4ta05294c

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We demonstrate a facile approach to fabricate Ag nanomesh transparent conducting electrodes (TCEs) on a flexible substrate using nanoimprint lithography (NIL) and transfer printing without a conducting polymer. The Ag nanomesh TCEs exhibited a high transmittance of similar to 88% and a low sheet resistance of similar to 15 Omega sq(-1) as well as superior mechanical flexibility. Furthermore, flexible inverted organic solar cells (IOSCs) with Ag nanomesh TCEs exhibited a power conversion efficiency (PCE) of similar to 7.15% under 100 mW cm (2) AM 1.5G illumination as well as superior long-term stability under ambient conditions. This type of highly flexible and transparent Ag nanomesh electrode is a promising candidate for use with TCEs in various optoelectronic devices.

引用

页码：65 / 70

页数：6

共 45 条

[1]

Bae S, 2010, NAT NANOTECHNOL, V5, P574, DOI [10.1038/nnano.2010.132, 10.1038/NNANO.2010.132]

[2] Flexible, Light-Weight, Ultrastrong, and Semiconductive Carbon Nanotube Fibers for a Highly Efficient Solar Cell [J].

Chen, Tao ;

Wang, Shutao ;

Yang, Zhibin ;

Feng, Quanyou ;

Sun, Xuemei ;

Li, Li ;

Wang, Zhong-Sheng ;

Peng, Huisheng .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2011, 50 (08) :1815-1819

[3] Silver Nanowire Networks as Flexible, Transparent, Conducting Films: Extremely High DC to Optical Conductivity Ratios [J].

De, Sukanta ;

Higgins, Thomas M. ;

Lyons, Philip E. ;

Doherty, Evelyn M. ;

Nirmalraj, Peter N. ;

Blau, Werner J. ;

Boland, John J. ;

Coleman, Jonathan N. .

ACS NANO, 2009, 3 (07) :1767-1774

[4]

Dressel M., 2002, Electrodynamics of Solids

[5] Smooth Nanowire/Polymer Composite Transparent Electrodes [J].

Gaynor, Whitney ;

Burkhard, George F. ;

McGehee, Michael D. ;

Peumans, Peter .

ADVANCED MATERIALS, 2011, 23 (26) :2905-2910

[6] Layer-by-Layer Doping of Few-Layer Graphene Film [J].

Gunes, Fethullah ;

Shin, Hyeon-Jin ;

Biswas, Chandan ;

Han, Gang Hee ;

Kim, Eun Sung ;

Chae, Seung Jin ;

Choi, Jae-Young ;

Lee, Young Hee .

ACS NANO, 2010, 4 (08) :4595-4600

[7]

He ZC, 2012, NAT PHOTONICS, V6, P591, DOI [10.1038/NPHOTON.2012.190, 10.1038/nphoton.2012.190]

[8] Nonvacuum, Maskless Fabrication of a Flexible Metal Grid Transparent Conductor by Low-Temperature Selective Laser Sintering of Nanoparticle Ink [J].

Hong, Sukjoon ;

Yeo, Junyeob ;

Kim, Gunho ;

Kim, Dongkyu ;

Lee, Habeom ;

Kwon, Jinhyeong ;

Lee, Hyungman ;

Lee, Phillip ;

Ko, Seung Hwan .

ACS NANO, 2013, 7 (06) :5024-5031

[9] Fast Inline Roll-to-Roll Printing for Indium-Tin-Oxide-Free Polymer Solar Cells Using Automatic Registration [J].

Hosel, Markus ;

Sondergaard, Roar R. ;

Jorgensen, Mikkel ;

Krebs, Frederik C. .

ENERGY TECHNOLOGY, 2013, 1 (01) :102-107

[10] Layer-by-Layer Graphene/TCNQ Stacked Films as Conducting Anodes for Organic Solar Cells [J].

Hsu, Chang-Lung ;

Lin, Cheng-Te ;

Huang, Jen-Hsien ;

Chu, Chih-Wei ;

Wei, Kung-Hwa ;

Li, Lain-Jong .

ACS NANO, 2012, 6 (06) :5031-5039

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