Anthropogenic pollutants in the Russian Arctic atmosphere: sources and sinks in spring and summer

The 5-day forward and backward trajectories of air mass transport to three Russian Arctic points for each day in April and July over a 10-year period from 1986 to 1995 have been analyzed. The important features and seasonal differences in air exchange processes in various areas of the Arctic have been investigated. Taking into account seasonal variations in aerosol scavenging mechanisms and velocities, the average contributions of large highly industrialized regions of the Russian Arctic air pollution were estimated for April and July. Reasonable correspondence between the calculated mean concentrations for six anthropogenic chemical elements (As, Ni, Pb, V, Zn, Cd) and experimentally determined values have been obtained. The atmospheric pollution transport from the Arctic was studied as yet another way of cleaning the Arctic atmosphere, in addition to the traditionally considered wet and dry depositions onto the surface. The average apportionment of conservative contaminants after passing the observation points was estimated for spring and summer. The air masses passing through the observation points in spring may take about 20-40% of pollutants out of the Arctic. In summer, however, more than 90% of pollutants transported into the Russian Arctic deposit within 5 days onto the surface inside the Arctic region. The monthly average fluxes of six anthropogenic elements onto the surface in the Russian Arctic were estimated for April and July. (C) 2000 Elsevier Science Ltd. All rights reserved.