Preparation of Magnetic Molecularly Imprinted Polymer (MMIP) Nanoparticles (NPs) for the Selective Extraction of Tetracycline from Milk

被引：24
作者：
Gao, Wanru [1 ]
Li, Jiayin [1 ]
Li, Pao [1 ]
Huang, Zhao [1 ]
Cao, Yanan [1 ]
Liu, Xia [1 ]
机构：
[1] Hunan Agr Univ, Hunan Prov Key Lab Food Sci & Biotechnol, Coll Food Sci & Technol, Changsha, Hunan, Peoples R China
来源：
ANALYTICAL LETTERS | 2020年 / 53卷 / 07期
基金：
中国国家自然科学基金;
关键词：
Magnetic molecularly imprinted polymer; selective adsorption; magnetic separation; tetracycline; milk; GREEN SYNTHESIS STRATEGY; SOLID-PHASE EXTRACTION; CARBON NANOTUBES; RECOGNITION; ANTIBIOTICS; CHLORAMPHENICOL; ADSORPTION; APTASENSOR; SEPARATION; ACRYLAMIDE;
D O I：
10.1080/00032719.2019.1698049
中图分类号：
O65 [分析化学];
学科分类号：
070302 ; 081704 ;
摘要：
Core-shell magnetic molecularly imprinted polymer nanoparticles (MMIP NPs) were prepared for the adsorption and the isolation of tetracycline from food matrices. The obtained MMIP NPs were characterized by transmission electron microscopy, Fourier transform infrared spectroscopy, X-ray diffractometry, vibrating sample magnetometry, and thermogravimetric analysis. The adsorption properties of the MMIP NPs were systematically characterized by static, kinetic, and selective adsorption as well as reusability measurements. The MMIP NPs were shown to provide a high adsorption capacity, with a maximum value of 40.48 mg/g, satisfactory selectivity with an imprinting factor equal to 2.55, and direct magnetic separation. Moreover, the MMIP NPs were successfully applied to extract tetracycline from milk samples. Satisfactory recoveries from 91.14 to 104.52% were obtained.
引用
收藏
页码：1097 / 1112
页数：16
相关论文
共 41 条
[1]   Dummy molecularly imprinted polymers based on a green synthesis strategy for magnetic solid-phase extraction of acrylamide in food samples [J].
Bagheri, Ahmad Reza ;
Arabi, Maryam ;
Ghaedi, Mehrorang ;
Ostovan, Abbas ;
Wang, Xiaoyan ;
Li, Jinhua ;
Chen, Lingxin .
TALANTA, 2019, 195 :390-400
[2]   Computational and experimental investigation of molecular imprinted polymers for selective extraction of dimethoate and its metabolite omethoate from olive oil [J].
Bakas, Idriss ;
Ben Oujji, Najwa ;
Moczko, Ewa ;
Istamboulie, Georges ;
Piletsky, Sergey ;
Piletska, Elena ;
Ait-Addi, Elhabib ;
Ait-Ichou, Ihya ;
Noguer, Thierry ;
Rouillon, Regis .
JOURNAL OF CHROMATOGRAPHY A, 2013, 1274 :13-18
[3]   ANALYSIS OF ACRYLAMIDE IN TRADITIONAL AND NONTRADITIONAL FOODS IN TURKEY USING HPLC-DAD WITH SPE CLEANUP [J].
Can, Nafiz Oncu ;
Arli, Goksel .
JOURNAL OF LIQUID CHROMATOGRAPHY & RELATED TECHNOLOGIES, 2014, 37 (06) :850-863
[4]   Development of a molecularly imprinted polymer for selective extraction of bisphenol A in water samples [J].
Canale, Francesca ;
Cordero, Chiara ;
Baggiani, Claudio ;
Baravalle, Patrizia ;
Giovannoli, Cristina ;
Bicchi, Carlo .
JOURNAL OF SEPARATION SCIENCE, 2010, 33 (11) :1644-1651
[5]   Analysis of volatile composition of siriguela (Spondias purpurea L.) by solid phase microextraction (SPME) [J].
Ceva-Antunes, PMN ;
Bizzo, HR ;
Silva, AS ;
Carvalho, CPS ;
Antunes, OAC .
LWT-FOOD SCIENCE AND TECHNOLOGY, 2006, 39 (04) :437-443
[6]   Magnetic molecularly imprinted polymer extraction of chloramphenicol from honey [J].
Chen, Ligang ;
Li, Bin .
FOOD CHEMISTRY, 2013, 141 (01) :23-28
[7]   Preparation of magnetic molecularly imprinted polymer for the separation of tetracycline antibiotics from egg and tissue samples [J].
Chen, Ligang ;
Liu, Jun ;
Zeng, Qinglei ;
Wang, Hui ;
Yu, Aimin ;
Zhang, Hanqi ;
Ding, Lan .
JOURNAL OF CHROMATOGRAPHY A, 2009, 1216 (18) :3710-3719
[8]   Molecular imprinting: perspectives and applications [J].
Chen, Lingxin ;
Wang, Xiaoyan ;
Lu, Wenhui ;
Wu, Xiaqing ;
Li, Jinhua .
CHEMICAL SOCIETY REVIEWS, 2016, 45 (08) :2137-2211
[9]   Recent advances in molecular imprinting technology: current status, challenges and highlighted applications [J].
Chen, Lingxin ;
Xu, Shoufang ;
Li, Jinhua .
CHEMICAL SOCIETY REVIEWS, 2011, 40 (05) :2922-2942
[10]   Versatile Method To Obtain Homogeneous Imprinted Polymer Thin Film at Surface of Superparamagnetic Nanoparticles for Tetracycline Binding [J].
Dai, Jiangdong ;
Zhou, Zhiping ;
Zhao, Chunyan ;
Wei, Xiao ;
Dai, Xiaohui ;
Gao, Lin ;
Cao, Zhijing ;
Yan, Yongsheng .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2014, 53 (17) :7157-7166
12345