Ionic liquids for high performance lithium metal batteries

被引：235
作者：
Liu, Kexin [1 ,2 ]
Wang, Zhuyi [2 ]
Shi, Liyi [2 ]
Jungsuttiwong, Siriporn [3 ,4 ]
Yuan, Shuai [2 ,5 ]
机构：
[1] Shanghai Univ, Sch Mat Sci & Engn, Shanghai 200444, Peoples R China
[2] Shanghai Univ, Res Ctr Nanosci & Nanotechnol, Shanghai 200444, Peoples R China
[3] Ubon Ratchathani Univ, Ctr Organ Elect & Alternat Energy, Dept Chem, Ubon Ratchathani 34190, Thailand
[4] Ubon Ratchathani Univ, Ctr Excellence Innovat Chem, Fac Sci, Ubon Ratchathani 34190, Thailand
[5] Shanghai Univ, Emerging Ind Inst, Jiaxing 314006, Zhejiang, Peoples R China
来源：
JOURNAL OF ENERGY CHEMISTRY | 2021年 / 59卷
基金：
中国国家自然科学基金;
关键词：
Ionic liquids; Li+ ion conduction; Interface issues; Lithium metal battery; SOLID POLYMER ELECTROLYTES; LI-S BATTERY; ELECTROCHEMICAL PROPERTIES; PYRROLIDINIUM CATIONS; RECHARGEABLE BATTERY; ENHANCED PERFORMANCE; THERMAL-PROPERTIES; INTERFACIAL LAYER; LI-O-2; BATTERIES; GEL ELECTROLYTE;
D O I：
10.1016/j.jechem.2020.11.017
中图分类号：
O69 [应用化学];
学科分类号：
081704 ;
摘要：
The pursuit of high energy density has promoted the development of high-performance lithium metal batteries. However, it faces a serious security problem. Ionic liquids have attracted great attention due to their high ionic conductivity, non-flammability, and the properties of promoting the formation of stable SEI films. Deeply understanding the problems existing in lithium metal batteries and the role of ionic liquids in them is of great significance for improving the performance of lithium metal batteries. This article reviews the effects of the molecular structure of ionic liquids on ionic conductivity, Li+ ion transference number, electrochemical stability window, and lithium metal anode/electrolyte interface, as well as the application of ionic liquids in Li-high voltage cathode batteries, Li-O-2 batteries and Li-S batteries. The molecular design, composition and polymerization will be the main strategies for the future development of ionic liquid-based electrolytes for high performance lithium metal battery. (C) 2020 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved.
引用
收藏
页码：320 / 333
页数：14
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