Potential Source Contribution Function Analysis of High Latitude Dust Sources over the Arctic: Preliminary Results and Prospects

被引:17
作者
Crocchianti, Stefano [1 ]
Moroni, Beatrice [1 ]
Waldhauserova, Pavla Dagsson [2 ,3 ]
Becagli, Silvia [4 ]
Severi, Mirko [4 ]
Traversi, Rita [4 ]
Cappelletti, David [1 ]
机构
[1] Univ Perugia, Dept Chem Biol & Biotechnol, I-06123 Perugia, Italy
[2] Agr Univ Iceland, Fac Environm & Forest Sci, IS-311 Hvanneyri, Iceland
[3] Czech Univ Life Sci Prague, Fac Environm Sci, Prague 16500, Czech Republic
[4] Univ Florence, Dept Chem, I-50019 Sesto Fiorentino, Italy
关键词
Svalbard; aerosol samples; back-trajectories; ICP-MS; mixing; emission;
D O I
10.3390/atmos12030347
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The results of a preliminary investigation of the dust sources in the Arctic based on their geochemical properties by potential source contribution function (PSCF) analysis are presented in this paper. For this purpose, we considered one year of aerosol geochemical data from Ny-angstrom lesund, Svalbard, and a short list of chemical elements (i.e., Al, Fe, Mn, Ti, Cr, V, Ni, Cu, and Zn) variably related to the dust fraction. Based on PSCF analysis: (i) four different dust source areas (i.e., Eurasia, Greenland, Arctic-Alaska, and Iceland) were characterized by distinguishing geochemical ranges and seasonal occurrence; and (ii) a series of typical dust days from the distinct source areas were identified based on the corresponding back trajectory patterns. Icelandic dust samples revealed peculiar but very variable characteristics in relation to their geographical source regions marked by air mass back trajectories. The comparison between pure and mixed Icelandic dust samples (i.e., aerosols containing Icelandic dust along with natural and/or anthropogenic components) revealed the occurrence of different mixing situations. Comparison with Icelandic soils proved the existence of dilution effects related to the emission and the transport processes.
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页数:15
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